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用于定制表面性能的AlCrFeMnTi高熵合金的露天大气压脉冲激光沉积的激光波长依赖性优化

Optimization of Laser-Wavelength Dependence for Open-Air Atmospheric Pressure Pulsed Laser Deposition of AlCrFeMnTi High-Entropy Alloy for Tailored Surface Properties.

作者信息

Mahdavi Hossein, Asghari Alamdari Armin, Kepceoğlu Abdullah, Yağcı M Barış, Ünal Uğur, Jahangiri Hadi

机构信息

Department of Materials Science and Engineering, Koç University, Sariyer 34450, Istanbul, Turkey.

Koç University Surface Science and Technology Center (KUYTAM), Koç University, Sariyer 34450, Istanbul, Turkey.

出版信息

ACS Omega. 2024 May 8;9(20):22495-22505. doi: 10.1021/acsomega.4c03245. eCollection 2024 May 21.

Abstract

High-entropy alloys (HEAs) have garnered significant attention in different fields due to their exceptional mechanical and physical properties, making them promising candidates for various applications. Several techniques, including physical vapor deposition and pulsed laser deposition (PLD), have been employed for the fabrication of HEA thin films. In this study, we explore a novel approach to synthesizing the lightweight HEA (LWHEA) AlCrFeMnTi using PLD in air at atmospheric pressure with a particular focus on the influence of the laser wavelength on the deposition process and the resulting alloy characteristics. This research investigates the impact of different laser wavelengths on the LWHEA's characterization and the optimization of laser wavelength dependence in air at atmospheric pressure PLD of LWHEA AlCrFeMnTi for tailored surface properties such as phase composition, microstructure, and corrosion resistance. Systematically varying the laser wavelength was attempted to optimize the deposition conditions. This was aimed at achieving enhanced properties and precise control over the alloy's composition. This work contributes to a deeper understanding of the open air PLD process for LWHEAs and sheds light on the role of the laser wavelength in tailoring their properties, which can have significant implications for the development of advanced materials for aerospace, automotive, and other high-performance applications. Ultimately, this research aims to provide valuable insights into the design and fabrication of LWHEAs with tailored properties through laser-based deposition techniques.

摘要

高熵合金(HEAs)因其优异的力学和物理性能在不同领域备受关注,使其成为各种应用的有前途的候选材料。包括物理气相沉积和脉冲激光沉积(PLD)在内的几种技术已被用于制备高熵合金薄膜。在本研究中,我们探索了一种在大气压力下于空气中使用脉冲激光沉积合成轻质高熵合金(LWHEA)AlCrFeMnTi的新方法,特别关注激光波长对沉积过程以及所得合金特性的影响。本研究调查了不同激光波长对LWHEA表征的影响,以及在大气压力下于空气中对LWHEA AlCrFeMnTi进行脉冲激光沉积时激光波长依赖性的优化,以实现诸如相组成、微观结构和耐腐蚀性等定制表面性能。尝试系统地改变激光波长以优化沉积条件。这旨在实现性能增强以及对合金成分的精确控制。这项工作有助于更深入地理解LWHEA在露天环境下的脉冲激光沉积过程,并揭示激光波长在定制其性能方面的作用,这对航空航天、汽车和其他高性能应用的先进材料开发可能具有重大意义。最终,本研究旨在通过基于激光的沉积技术为具有定制性能的LWHEA的设计和制造提供有价值的见解。

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