Chacon Reinaldo, Leray Aymeric, Kim Jeongmo, Lahlil Khalid, Bouhelier Alexandre, Kim Jong-Wook, Gacoin Thierry, Colas des Francs Gérard
Laboratoire Interdisciplinaire Carnot de Bourgogne (ICB), UMR 6303 CNRS, Université Bourgogne-Franche-Comté, 9 Avenue Savary, BP 47870, F-21078 Dijon Cedex, France.
Physique de la Matière Condensée, CNRS UMR 7643, Ecole Polytechnique, F-91128 Palaiseau, France.
Nanotechnology. 2022 Jul 1;33(38). doi: 10.1088/1361-6528/ac7884.
We use europium doped single crystalline NaYFnanorods for probing the electric and magnetic contributions to the local density of optical states (LDOS). Reciprocically, we determine intrinsic properties of the emitters (oscillator strength, quantum yield) by comparing their measured and simulated optical responses in front of a mirror. We first experimentally determine the specifications of the nanoprobe (orientation and oscillator strength of the electric and magnetic dipoles moments) and show significant orientation sensitivity of the branching ratios associated with electric and magnetic transitions. In a second part, we measure the modification of the LDOS in front of a gold mirror in a Drexhage's experiment. We discuss the role of the electric and magnetic LDOS on the basis of numerical simulations, taking into account the orientation of the dipolar emitters. We demonstrate that they behave like degenerated dipoles sensitive to polarized partial LDOS.
我们使用铕掺杂的单晶NaYF纳米棒来探测对光学态局域密度(LDOS)的电和磁贡献。相反,我们通过比较发射体在镜子前的测量和模拟光学响应来确定其固有特性(振子强度、量子产率)。我们首先通过实验确定纳米探针的规格(电偶极矩和磁偶极矩的取向和振子强度),并表明与电和磁跃迁相关的分支比具有显著的取向敏感性。在第二部分中,我们在德雷夏格实验中测量了金镜前LDOS的变化。我们基于数值模拟讨论电和磁LDOS的作用,同时考虑偶极发射体的取向。我们证明它们的行为类似于对极化部分LDOS敏感的简并偶极子。