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时域中光学态局部密度的直接测量。

Direct Measurement of the Local Density of Optical States in the Time Domain.

作者信息

Ter Huurne Stan E T, Peeters Djero B L, Sánchez-Gil Jose A, Rivas Jaime Gómez

机构信息

Department of Applied Physics and Science Education, and Eindhoven Hendrik Casimir Institute, Eindhoven University of Technology, P.O. Box 513, Eindhoven 5600 MB, The Netherlands.

Instituto de Estructura de La Materia, Consejo Superior de Investigaciones Científicas (IEM-CSIC), Serrano 121, Madrid 28006, Spain.

出版信息

ACS Photonics. 2023 Aug 1;10(8):2980-2986. doi: 10.1021/acsphotonics.3c00781. eCollection 2023 Aug 16.

Abstract

One of the most fundamental and relevant properties of a photonic system is the local density of optical states (LDOS) as it defines the rate at which an excited emitter dissipates energy by coupling to its surrounding. However, the direct determination of the LDOS is challenging as it requires measurements of the complex electric field of a point dipole at its own position. We introduce here a near-field setup which can measure the terahertz electric field amplitude at the position of a point source in the time domain. From the measured amplitude, the frequency-dependent imaginary component of the electric field can be determined and the LDOS can be retrieved. As a proof of concept, this setup has been used to measure the partial LDOS (the LDOS for a defined dipole orientation) as a function of the distance to planar interfaces made of gold, InSb, and quartz. Furthermore, the spatially dependent partial LDOS of a resonant gold rod has been measured as well. These results have been compared with analytical results and simulations. The excellent agreement between measurements and theory demonstrates the applicability of this setup for the quantitative determination of the LDOS in complex photonic systems.

摘要

光子系统最基本且相关的特性之一是光态密度(LDOS),因为它决定了受激发射体通过与周围环境耦合而耗散能量的速率。然而,直接确定LDOS具有挑战性,因为这需要在点偶极子自身位置测量其复电场。我们在此介绍一种近场装置,它可以在时域中测量点源位置处的太赫兹电场幅度。根据测量的幅度,可以确定电场的频率相关虚部,并可以检索到LDOS。作为概念验证,该装置已用于测量部分LDOS(定义偶极子方向的LDOS)作为到由金、锑化铟和石英制成的平面界面距离的函数。此外,还测量了共振金棒的空间相关部分LDOS。这些结果已与分析结果和模拟进行了比较。测量结果与理论之间的出色一致性证明了该装置在复杂光子系统中定量确定LDOS的适用性。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/c1aa/10436706/d8df16fcc1c0/ph3c00781_0002.jpg

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