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利用圆柱矢量光束控制与硅纳米天线耦合的量子发射器的光发射。

Control of light emission of quantum emitters coupled to silicon nanoantenna using cylindrical vector beams.

作者信息

Montagnac Martin, Brûlé Yoann, Cuche Aurélien, Poumirol Jean-Marie, Weber Sébastien J, Müller Jonas, Larrieu Guilhem, Larrey Vincent, Fournel Franck, Boisron Olivier, Masenelli Bruno, Colas des Francs Gérard, Agez Gonzague, Paillard Vincent

机构信息

CEMES-CNRS, Université de Toulouse, Toulouse, France.

ICB, Université de Bourgogne, CNRS, Dijon, France.

出版信息

Light Sci Appl. 2023 Sep 19;12(1):239. doi: 10.1038/s41377-023-01229-9.

Abstract

Light emission of europium (Eu) ions placed in the vicinity of optically resonant nanoantennas is usually controlled by tailoring the local density of photon states (LDOS). We show that the polarization and shape of the excitation beam can also be used to manipulate light emission, as azimuthally or radially polarized cylindrical vector beam offers to spatially shape the electric and magnetic fields, in addition to the effect of silicon nanorings (Si-NRs) used as nanoantennas. The photoluminescence (PL) mappings of the Eu transitions and the Si phonon mappings are strongly dependent of both the excitation beam and the Si-NR dimensions. The experimental results of Raman scattering and photoluminescence are confirmed by numerical simulations of the near-field intensity in the Si nanoantenna and in the Eu-doped film, respectively. The branching ratios obtained from the experimental PL maps also reveal a redistribution of the electric and magnetic emission channels. Our results show that it could be possible to spatially control both electric and magnetic dipolar emission of Eu ions by switching the laser beam polarization, hence the near field at the excitation wavelength, and the electric and magnetic LDOS at the emission wavelength. This paves the way for optimized geometries taking advantage of both excitation and emission processes.

摘要

置于光学共振纳米天线附近的铕(Eu)离子的发光通常通过调整光子态密度(LDOS)来控制。我们表明,激发光束的偏振和形状也可用于操纵发光,因为方位角或径向偏振的圆柱矢量光束除了用作纳米天线的硅纳米环(Si-NRs)的作用外,还能在空间上塑造电场和磁场。Eu跃迁的光致发光(PL)映射和Si声子映射强烈依赖于激发光束和Si-NR尺寸。拉曼散射和光致发光的实验结果分别通过Si纳米天线和Eu掺杂薄膜中近场强度的数值模拟得到证实。从实验PL图获得的分支比还揭示了电发射和磁发射通道的重新分布。我们的结果表明,通过切换激光束偏振,从而改变激发波长处的近场以及发射波长处的电和磁LDOS,有可能在空间上控制Eu离子的电偶极和磁偶极发射。这为利用激发和发射过程的优化几何结构铺平了道路。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/db4f/10509260/e0f6a5c51fba/41377_2023_1229_Fig1_HTML.jpg

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