State Environmental Protection Key Laboratory of Urban Ambient Air Particulate Matter Pollution Prevention and Control & Tianjin Key Laboratory of Urban Transport Emission Research, College of Environmental Science and Engineering, Nankai University, Tianjin, 300350, China.
State Environmental Protection Key Laboratory of Urban Ambient Air Particulate Matter Pollution Prevention and Control & Tianjin Key Laboratory of Urban Transport Emission Research, College of Environmental Science and Engineering, Nankai University, Tianjin, 300350, China.
Environ Pollut. 2021 Sep 1;284:117454. doi: 10.1016/j.envpol.2021.117454. Epub 2021 May 23.
Levels of toxic elements in ambient PM were measured from 29 October 2019 to 30 March 2020 in Linfen, China, to assess the health risks they posed and to identify critical risk sources during different periods of the COVID-19 lockdown and haze episodes using positive matrix factorization (PMF) and a health-risk assessment model. The mean PM concentration during the study period was 145 μg/m, and the 10 investigated toxic elements accounted for 0.31% of the PM mass. The total non-cancer risk (HI) and total cancer risk (TCR) of the selected toxic elements exceed the US EPA limits for children and adults. The HI for children was 2.3 times that for adults for all periods, which is likely due to the high inhalation rate per unit body weight for children. While the TCR for adults was 1.7 times that of children, which is mainly attributed to potential longer exposure duration for adults. The HI and TCR of the toxic elements during full lockdown were reduced by 66% and 58%, respectively, compared to their pre-lockdown levels. The HI and TCR were primarily attributable to Mn and As, respectively. Health risks during haze episodes were significantly higher than the average levels during COVID-19 lockdowns, though the HI and TCR of the selected toxic elements during full-lockdown haze episodes were 68% and 17% lower, respectively, than were the levels during pre-lockdown haze episodes. During the study period, fugitive dust and steel-related smelting were the highest contributors to HI and TCR, respectively, and decreased in these emission sources contributed the most to the lower health risks observed during the full lockdown. There, the control of these sources is critical to effectively reduce public health risks.
2019 年 10 月 29 日至 2020 年 3 月 30 日,在中国临汾测量了环境 PM 中的有毒元素水平,以评估它们在 COVID-19 封锁和雾霾期间不同时期构成的健康风险,并利用正定矩阵因子分解 (PMF) 和健康风险评估模型识别关键风险源。研究期间的 PM 平均浓度为 145μg/m,所研究的 10 种有毒元素占 PM 质量的 0.31%。所选有毒元素的非癌症总风险 (HI) 和总癌症风险 (TCR) 超过了美国环保署对儿童和成人的限值。所有时期儿童的 HI 均是成人的 2.3 倍,这可能是由于儿童单位体重的吸入率较高。而成年人的 TCR 是儿童的 1.7 倍,这主要归因于成年人潜在的更长暴露时间。与封锁前相比,全面封锁期间有毒元素的 HI 和 TCR 分别降低了 66%和 58%。HI 和 TCR 主要归因于 Mn 和 As。雾霾期间的健康风险明显高于 COVID-19 封锁期间的平均水平,尽管全面封锁雾霾期间的 HI 和 TCR 分别比封锁前雾霾期间低 68%和 17%。在研究期间,扬尘和与钢铁相关的冶炼分别是 HI 和 TCR 的最大贡献者,这些排放源的减少对观察到的全面封锁期间较低的健康风险贡献最大。在那里,控制这些来源对于有效降低公共健康风险至关重要。