Zhang Minna, Xuan Xiaoxu, Yi Xibin, Sun Jinqiang, Wang Mengjie, Nie Yihao, Zhang Jing, Sun Xun
Shandong Key Laboratory for Special Silicon-Containing Material, Advanced Materials Institute, Qilu University of Technology (Shandong Academy of Sciences), Jinan 250014, China.
Key Laboratory of High Efficiency and Clean Mechanical Manufacture, Ministry of Education, School of Mechanical Engineering, Shandong University, Jinan 250061, China.
Nanomaterials (Basel). 2022 Aug 8;12(15):2721. doi: 10.3390/nano12152721.
Carbon aerogel (CA) based materials have multiple advantages, including high porosity, tunable molecular structures, and environmental compatibility. Increasing interest, which has focused on CAs as electrocatalysts for sustainable applications including oxygen reduction reaction (ORR), oxygen evolution reaction (OER), hydrogen evolution reaction (HER), and CO reduction reaction (CORR) has recently been raised. However, a systematic review covering the most recent progress to boost CA-based electrocatalysts for ORR/OER/HER/CORR is now absent. To eliminate the gap, this critical review provides a timely and comprehensive summarization of the applications, synthesis methods, and principles. Furthermore, prospects for emerging synthesis, screening, and construction methods are outlined.
基于碳气凝胶（CA）的材料具有多种优势，包括高孔隙率、可调节的分子结构以及环境兼容性。近来，人们对碳气凝胶作为可持续应用的电催化剂的兴趣日益浓厚，这些应用包括氧还原反应（ORR）、析氧反应（OER）、析氢反应（HER）和一氧化碳还原反应（CORR）。然而，目前缺乏对用于ORR/OER/HER/CORR的基于CA的电催化剂的最新进展的系统综述。为了消除这一差距，本综述及时全面地总结了其应用、合成方法和原理。此外，还概述了新兴合成、筛选和构建方法的前景。
