Chen Lu, Boulanger Marie-Eve, Wang Zhi-Cheng, Tafti Fazel, Taillefer Louis
Département de Physique, Institut Quantique and Regroupement Québécois sur les Matériaux de Pointe, Université de Sherbrooke, Sherbrooke, QC J1K 2R1, Canada.
Department of Physics, Boston College, Chestnut Hill, MA 02467.
Proc Natl Acad Sci U S A. 2022 Aug 23;119(34):e2208016119. doi: 10.1073/pnas.2208016119. Epub 2022 Aug 15.
Phonons are known to generate a thermal Hall effect in certain insulators, including oxides with rare-earth impurities, quantum paraelectrics, multiferroic materials, and cuprate Mott insulators. In each case, a special feature of the material is presumed relevant for the underlying mechanism that confers chirality to phonons in a magnetic field. A fundamental question is whether a phonon Hall effect is an unusual occurrence-linked to special characteristics such as skew scattering off rare-earth impurities, structural domains, ferroelectricity, or ferromagnetism-or a much more common property of insulators than hitherto believed. To help answer this question, we have turned to a material with none of the previously encountered special features: the cubic antiferromagnet CuTeO. We find that its thermal Hall conductivity [Formula: see text] is among the largest of any insulator so far. We show that this record-high [Formula: see text] signal is due to phonons, and it does not require the presence of magnetic order, as it persists above the ordering temperature. We conclude that the phonon Hall effect is likely to be a fairly common property of solids.
已知声子会在某些绝缘体中产生热霍尔效应,这些绝缘体包括含有稀土杂质的氧化物、量子顺电体、多铁性材料和铜酸盐莫特绝缘体。在每种情况下,人们认为材料的一个特殊特征与在磁场中赋予声子手性的潜在机制有关。一个基本问题是,声子霍尔效应是一种与诸如稀土杂质的斜散射、结构域、铁电性或铁磁性等特殊特征相关的罕见现象,还是比迄今所认为的更常见的绝缘体属性。为了帮助回答这个问题,我们转向了一种没有上述任何特殊特征的材料:立方反铁磁体CuTeO。我们发现其热霍尔电导率[公式:见正文]是迄今为止所有绝缘体中最大的之一。我们表明,这个创纪录的高[公式:见正文]信号是由声子引起的,并且它不需要磁有序的存在,因为它在有序温度以上仍然存在。我们得出结论,声子霍尔效应可能是固体中相当普遍的属性。