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对硒这一新兴污染物的来源、污染及修复的批判性分析。

A critical analysis of sources, pollution, and remediation of selenium, an emerging contaminant.

机构信息

Department of Environmental Science, Zhejiang University, Hangzhou, 310058, Zhejiang, China.

Zhejiang Provincial Key Laboratory of Organic Pollutant Process and Control, Zhejiang University, Hangzhou, 310058, Zhejiang, China.

出版信息

Environ Geochem Health. 2023 May;45(5):1359-1389. doi: 10.1007/s10653-022-01354-1. Epub 2022 Aug 16.

Abstract

Selenium (Se) is an essential metalloid and is categorized as emerging anthropogenic contaminant released to the environment. The rise of Se release into the environment has raised concern about its bioaccumulation, toxicity, and potential to cause serious damages to aquatic and terrestrial ecosystem. Therefore, it is extremely important to monitor Se level in environment on a regular basis. Understanding Se release, anthropogenic sources, and environmental behavior is critical for developing an effective Se containment strategy. The ongoing efforts of Se remediation have mostly emphasized monitoring and remediation as an independent topics of research. However, our paper has integrated both by explaining the attributes of monitoring on effective scale followed by a candid review of widespread technological options available with specific focus on Se removal from environmental media. Another novel approach demonstrated in the article is the presentation of an overwhelming evidence of limitations that various researchers are confronted with to overcome achieving effective remediation. Furthermore, we followed a holistic approach to discuss ways to remediate Se for cleaner environment especially related to introducing weak magnetic field for ZVI reactivity enhancement. We linked this phenomenal process to electrokinetics and presented convincing facts in support of Se remediation, which has led to emerge 'membrane technology', as another viable option for remediation. Hence, an interesting, innovative and future oriented review is presented, which will undoubtedly seek attention from global researchers.

摘要

硒(Se)是一种必需的类金属,被归类为新兴的人为污染物,释放到环境中。硒向环境中的释放增加引起了人们对其生物累积、毒性以及对水生和陆地生态系统造成严重损害的潜力的关注。因此,定期监测环境中的硒水平非常重要。了解硒的释放、人为来源和环境行为对于制定有效的硒控制策略至关重要。目前,硒修复的工作主要侧重于监测和修复作为独立的研究课题。然而,我们的论文通过解释有效规模监测的属性,并对广泛可用的技术选择进行坦率的回顾,将两者结合在一起,重点是从环境介质中去除硒。本文还展示了一种新颖的方法,即展示了各种研究人员在实现有效修复方面所面临的限制的压倒性证据。此外,我们还采用了整体方法来讨论修复硒以实现更清洁环境的方法,特别是引入弱磁场以增强零价铁的反应性。我们将这一现象过程与电动学联系起来,并提出了令人信服的事实来支持硒的修复,这导致了“膜技术”作为另一种可行的修复选择的出现。因此,本文提出了一篇有趣、创新和面向未来的综述,无疑将引起全球研究人员的关注。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/5812/9379879/7412bf3c58e8/10653_2022_1354_Fig1_HTML.jpg

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