Nicolas Alexandre, Rottler Jörg, Barrat Jean-Louis
LIPhy, Univ. Grenoble Alpes, F-38000, Grenoble, France,
Eur Phys J E Soft Matter. 2014 Jun;37(6):9. doi: 10.1140/epje/i2014-14050-1. Epub 2014 Jun 26.
The slow flow of amorphous solids exhibits striking heterogeneities: swift localised particle rearrangements take place in the midst of a more or less homogeneously deforming medium. Recently, experimental as well as numerical work has revealed spatial correlations between these flow heterogeneities. Here, we use molecular dynamics (MD) simulations to characterise the rearrangements and systematically probe their correlations both in time and in space. In particular, these correlations display a four-fold azimuthal symmetry characteristic of shear stress redistribution in an elastic medium and we unambiguously detect their increase in range with time. With increasing shear rate, correlations become shorter-ranged. In addition, we study a coarse-grained model motivated by the observed flow characteristics and challenge its predictions directly with the MD simulations. While the model captures both macroscopic and local properties rather satisfactorily, the agreement with respect to the spatiotemporal correlations is at most qualitative. The discrepancies provide important insight into relevant physics that is missing in all related coarse-grained models that have been developed for the flow of amorphous materials so far, namely the finite shear wave velocity and the impact of elastic heterogeneities on stress redistribution.
在或多或少均匀变形的介质中会发生快速的局部粒子重排。最近,实验和数值研究工作揭示了这些流动不均匀性之间的空间相关性。在此,我们使用分子动力学(MD)模拟来表征重排,并系统地探究它们在时间和空间上的相关性。特别地,这些相关性呈现出弹性介质中剪切应力重新分布所特有的四重方位对称性,并且我们明确检测到它们的范围随时间增加。随着剪切速率的增加,相关性的范围变短。此外,我们研究了一个受观测到的流动特性驱动的粗粒化模型,并直接用MD模拟对其预测进行检验。虽然该模型相当令人满意地捕捉了宏观和局部特性,但在时空相关性方面的一致性最多只是定性的。这些差异为所有目前已开发的用于非晶态材料流动的相关粗粒化模型中所缺失的相关物理提供了重要见解,即有限的剪切波速度以及弹性不均匀性对应力重新分布的影响。