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Kagome磁体FeSn中反铁磁结构的自旋极化成像及场可调束缚态

Spin-polarized imaging of the antiferromagnetic structure and field-tunable bound states in kagome magnet FeSn.

作者信息

Li Hong, Zhao He, Yin Qiangwei, Wang Qi, Ren Zheng, Sharma Shrinkhala, Lei Hechang, Wang Ziqiang, Zeljkovic Ilija

机构信息

Department of Physics, Boston College, Chestnut Hill, MA, 02467, USA.

Department of Physics and Beijing Key Laboratory of Opto-Electronic Functional Materials & Micro-Nano Devices, Renmin University of China, Beijing, 100872, China.

出版信息

Sci Rep. 2022 Aug 25;12(1):14525. doi: 10.1038/s41598-022-18678-8.

Abstract

Kagome metals are an exciting playground for the explorations of novel phenomena at the intersection of topology, electron correlations and magnetism. The family of FeSn-based kagome magnets in particular attracted a lot of attention for simplicity of the layered crystal structure and tunable topological electronic band structure. Despite a significant progress in understanding their bulk properties, surface electronic and magnetic structures are yet to be fully explored in many of these systems. In this work, we focus on a prototypical kagome metal FeSn. Using a combination of spin-averaged and spin-polarized scanning tunneling microscopy, we provide the first atomic-scale visualization of the layered antiferromagnetic structure at the surface of FeSn. In contrast to the field-tunable electronic structure of cousin material FeSn that is a ferromagnet, we find that electronic density-of-states of FeSn is robust to the application of external magnetic field. Interestingly, despite the field insensitive electronic band structure, FeSn exhibits bound states tied to specific impurities with large effective moments that strongly couple to the magnetic field. Our experiments provide microscopic insights necessary for theoretical modeling of FeSn and serve as a spring board for spin-polarized measurements of topological magnets in general.

摘要

Kagome金属是拓扑学、电子关联和磁性交叉领域探索新现象的一个令人兴奋的研究平台。特别是基于FeSn的Kagome磁体家族,因其层状晶体结构的简单性和可调节的拓扑电子能带结构而备受关注。尽管在理解它们的体性质方面取得了重大进展,但在许多这类体系中,表面电子和磁性结构仍有待充分探索。在这项工作中,我们聚焦于典型的Kagome金属FeSn。通过结合自旋平均和自旋极化扫描隧道显微镜,我们首次在原子尺度上可视化了FeSn表面的层状反铁磁结构。与同为铁磁体的同类材料FeSn的场可调电子结构不同,我们发现FeSn的电子态密度对外加磁场的应用具有鲁棒性。有趣的是,尽管电子能带结构对磁场不敏感,但FeSn表现出与具有大有效磁矩的特定杂质相关的束缚态,这些束缚态与磁场强烈耦合。我们的实验为FeSn的理论建模提供了必要的微观见解,并总体上为拓扑磁体的自旋极化测量提供了一个跳板。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/4c50/9411549/e503935a4772/41598_2022_18678_Fig1_HTML.jpg

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