South China Institute of Environmental Sciences, Ministry of Ecology and Environment, Guangzhou, 510535, China.
SCNU Environmental Research Institute, Guangdong Provincial Key Laboratory of Chemical Pollution and Environmental Safety & MOE Key Laboratory of Theoretical Chemistry of Environment, South China Normal University, 510006, Guangzhou, China; School of Environment, South China Normal University, University Town, 510006, Guangzhou, China.
Chemosphere. 2022 Dec;308(Pt 2):136252. doi: 10.1016/j.chemosphere.2022.136252. Epub 2022 Aug 30.
Characterising the daily PM2.5 concentration is crucial for air quality control. To govern the status of the atmospheric environment, a novel hybrid model for PM2.5 forecasting was proposed by introducing a two-stage decomposition technology of complete ensemble empirical mode decomposition with adaptive noise (CEEMDAN) and variational mode decomposition (VMD); subsequently, a deep learning approach of long short-term memory (LSTM) was proposed. Five cities with unique meteorological and economic characteristics were selected to assess the predictive ability of the proposed model. The results revealed that PM2.5 pollution was generally more severe in inland cities (66.98 ± 0.76 μg m) than in coastal cities (40.46 ± 0.40 μg m-3). The modelling comparison showed that in each city, the secondary decomposition algorithm improved the accuracy and prediction stability of the prediction models. When compared with other prediction models, LSTM effectively extracted featured information and achieved relatively accurate time-series prediction. The hybrid model of CEEMDAN-VMD-LSTM achieved a better prediction in the five cities (R2 = 0.9803 ± 0.01) compared with the benchmark models (R2 = 0.7537 ± 0.03). The results indicate that the proposed approach can identify the inherent correlations and patterns among complex datasets, particularly in time-series analysis.
描述每日 PM2.5 浓度对于空气质量控制至关重要。为了治理大气环境状况,本文提出了一种新颖的混合模型,该模型通过引入完全集合经验模态分解与自适应噪声(CEEMDAN)和变分模态分解(VMD)的两阶段分解技术,以及长短期记忆(LSTM)的深度学习方法来进行 PM2.5 预测。选择了五个具有独特气象和经济特征的城市来评估所提出模型的预测能力。结果表明,内陆城市的 PM2.5 污染一般比沿海城市(66.98±0.76μg m-3)更为严重(40.46±0.40μg m-3)。模型比较表明,在每个城市中,二次分解算法提高了预测模型的准确性和预测稳定性。与其他预测模型相比,LSTM 有效地提取了特征信息,并实现了相对准确的时间序列预测。CEEMDAN-VMD-LSTM 混合模型在五个城市中的预测效果优于基准模型(R2=0.9803±0.01,R2=0.7537±0.03)。结果表明,所提出的方法可以识别复杂数据集之间的内在相关性和模式,尤其是在时间序列分析中。