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重氪离子和氙离子辐照下 WO 微粒的抗辐射性研究

Study of Radiation Resistance of WO Microparticles under Irradiation with Heavy Kr and Xe Ions.

作者信息

Kadyrzhanov Dauren B, Kozlovskiy Artem L, Zdorovets Maxim V, Khametova Ainagul A, Shlimas Dmitriy I

机构信息

Engineering Profile Laboratory, L.N. Gumilyov Eurasian National University, Nur-Sultan 010008, Kazakhstan.

Laboratory of Solid State Physics, The Institute of Nuclear Physics, Almaty 050032, Kazakhstan.

出版信息

Nanomaterials (Basel). 2022 Aug 24;12(17):2909. doi: 10.3390/nano12172909.

Abstract

In this work, we consider the effect of irradiation with heavy Kr and Xe ions on the change in the structural and strength properties of WO microparticles, which are among the candidates for inert matrix materials. Irradiation with heavy Kr and Xe ions was chosen to determine the possibility of simulation of radiation damage comparable to the impact of fission fragments. During the studies, it was found that the main changes in the structural properties with an increase in the irradiation fluence are associated with the crystal lattice deformation and its anisotropic distortion, which is most pronounced during irradiation with heavy Kr ions. An assessment of the gaseous swelling effect due to the radiation damage accumulation showed that a change in the ion type during irradiation leads to an increase in the swelling value by more than 8-10%. Results of strength changes showed that the most intense decrease in the hardness of the near-surface layer is observed when the fluence reaches more than 10 ion/cm, which is typical for the effect of overlapping radiation damage in the material. The dependences obtained for the change in structural and strength properties can later be used to evaluate the effectiveness of the use of refractory oxide materials for their use in the creation of inert matrices of nuclear fuel.

摘要

在这项工作中,我们考虑了用重氪离子和氙离子辐照对WO微粒结构和强度性能变化的影响,WO微粒是惰性基体材料的候选材料之一。选择用重氪离子和氙离子辐照,以确定模拟与裂变碎片影响相当的辐射损伤的可能性。在研究过程中发现,随着辐照注量增加,结构性能的主要变化与晶格变形及其各向异性畸变有关,这在重氪离子辐照期间最为明显。对由于辐射损伤积累导致的气体肿胀效应的评估表明,辐照期间离子类型的变化会使肿胀值增加超过8 - 10%。强度变化结果表明,当注量超过10离子/cm²时,观察到近表面层硬度最剧烈下降,这是材料中辐射损伤重叠效应的典型情况。所获得的结构和强度性能变化的相关性,稍后可用于评估难熔氧化物材料在用于制造核燃料惰性基体方面的使用效果。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/5bb6/9458222/0aafe2ac6b3f/nanomaterials-12-02909-g001.jpg

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