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重离子辐照下CeO陶瓷中辐射损伤动力学的研究

Study of the Kinetics of Radiation Damage in CeO Ceramics upon Irradiation with Heavy Ions.

作者信息

Giniyatova Sholpan G, Kozlovskiy Artem L, Rspayev Ruslan M, Borgekov Daryn B, Zdorovets Maxim V

机构信息

Engineering Profile Laboratory, L.N. Gumilyov Eurasian National University, Satpayev St., Astana 010008, Kazakhstan.

Department of General Physics, Satbayev University, Almaty 050032, Kazakhstan.

出版信息

Materials (Basel). 2023 Jun 28;16(13):4653. doi: 10.3390/ma16134653.

Abstract

In this work, the effect of irradiation with heavy Kr and Xe ions on the change in the structural and strength properties of CeO microstructural ceramics, which is one of the candidates for inert matrix materials for dispersed nuclear fuel, is considered. Irradiation with heavy Kr and Xe ions was chosen to determine the possibility of simulation of radiation damage comparable to the action of fission fragments, as well as neutron radiation, considering damage accumulation at a given depth of the near-surface layer. During the research, it was found that the main changes in the structural properties with an increase in the irradiation fluence are associated with the crystal lattice deformation distortions and the consequent radiation damage accumulation in the surface layer, and its swelling. Evaluation of the effect of gaseous swelling caused by the radiation damage accumulation showed that a variation in the ion type during irradiation results in a growth in the value of swelling and destruction of the near-surface layer with the accumulation of deformation distortions. Results of the strength variation demonstrated that the most intense decrease in the near-surface layer hardness is observed when the fluence reaches more than 10-10 ion/cm, which is typical for the effect of overlapping radiation damage in the material.

摘要

在这项工作中,考虑了用重氪离子和氙离子辐照对CeO微结构陶瓷结构和强度性能变化的影响,CeO微结构陶瓷是分散核燃料惰性基体材料的候选材料之一。选择用重氪离子和氙离子辐照,以确定模拟与裂变碎片作用以及中子辐射相当的辐射损伤的可能性,同时考虑近表层给定深度处的损伤积累。在研究过程中发现,随着辐照通量的增加,结构性能的主要变化与晶格变形畸变以及随之而来的表层辐射损伤积累及其肿胀有关。对由辐射损伤积累引起的气体肿胀效应的评估表明,辐照过程中离子类型的变化会导致肿胀值增加以及近表层因变形畸变积累而破坏。强度变化结果表明,当通量超过10^10离子/cm²时,近表层硬度下降最为剧烈,这是材料中辐射损伤重叠效应的典型表现。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/7411/10342356/e3a3ba951dbe/materials-16-04653-g001.jpg

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