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通过光子束内外的光学束缚形成的原始光学演化物质。

The primeval optical evolving matter by optical binding inside and outside the photon beam.

作者信息

Huang Chih-Hao, Louis Boris, Bresolí-Obach Roger, Kudo Tetsuhiro, Camacho Rafael, Scheblykin Ivan G, Sugiyama Teruki, Hofkens Johan, Masuhara Hiroshi

机构信息

Department of Applied Chemistry, College of Science, National Yang Ming Chiao Tung University, Hsinchu, 30010, Taiwan.

Laboratory for Photochemistry and Spectroscopy, Division for Molecular Imaging and Photonics, Department of Chemistry, Katholieke Universiteit Leuven, Leuven, 3001, Belgium.

出版信息

Nat Commun. 2022 Sep 10;13(1):5325. doi: 10.1038/s41467-022-33070-w.

Abstract

Optical binding has recently gained considerable attention because it enables the light-induced assembly of many-body systems; however, this phenomenon has only been described between directly irradiated particles. Here, we demonstrate that optical binding can occur outside the focal spot of a single tightly focused laser beam. By trapping at an interface, we assemble up to three gold nanoparticles with a linear arrangement which fully-occupies the laser focus. The trapping laser is efficiently scattered by this linear alignment and interacts with particles outside the focus area, generating several discrete arc-shape potential wells with a half-wavelength periodicity. Those external nanoparticles inside the arcs show a correlated motion not only with the linear aligned particles, but also between themselves even both are not directly illuminated. We propose that the particles are optically bound outside the focal spot by the back-scattered light and multi-channel light scattering, forming a dynamic optical binding network.

摘要

光学束缚最近受到了广泛关注,因为它能够实现光诱导的多体系统组装;然而,这种现象仅在直接照射的粒子之间被描述过。在这里,我们证明光学束缚可以发生在单个紧聚焦激光束的焦斑之外。通过在界面处捕获,我们组装了多达三个呈线性排列的金纳米粒子,这种排列完全占据了激光焦点。捕获激光被这种线性排列有效地散射,并与焦点区域外的粒子相互作用,产生几个具有半波长周期性的离散弧形势阱。这些弧形内的外部纳米粒子不仅与线性排列的粒子表现出相关运动,而且即使它们都没有被直接照射,彼此之间也表现出相关运动。我们提出,粒子通过背向散射光和多通道光散射在焦斑外被光学束缚,形成一个动态光学束缚网络。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a64a/9464242/aabac7befe5b/41467_2022_33070_Fig1_HTML.jpg

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