Morita Yusuke, Yoshioka Kosuke, Kuwata-Gonokami Makoto
Department of Physics, Graduate School of Science, The University of Tokyo, 7-3-1 Hongo, Bunkyo-ku, Tokyo, 113-0033, Japan.
Photon Science Center, Graduate School of Engineering, The University of Tokyo, 2-11-16 Yayoi, Bunkyo-ku, Tokyo, 113-8656, Japan.
Nat Commun. 2022 Sep 14;13(1):5388. doi: 10.1038/s41467-022-33103-4.
An unambiguous observation of the Bose-Einstein condensation (BEC) of excitons in a photoexcited bulk semiconductor and elucidation of its inherent nature have been longstanding problems in condensed matter physics. Here, we observe the quantum phase transition and a Bose-Einstein condensate appearing in a trapped gas of 1s paraexcitons in bulk CuO below 400 mK, by directly visualizing the exciton cloud in real space using mid-infrared induced absorption imaging that we realized in a dilution refrigerator. Our study shows that the paraexciton condensate is undetectable by conventional luminescence spectroscopy. We find an unconventionally small condensate fraction of 0.016 with the spatial profile of the condensate well described by mean-field theory. Our discovery of this new type of BEC in the purely matter-like exciton system interacting with a cold phonon bath could pave the way for the classification of its long-range order, and for essential understanding of quantum statistical mechanics of non-equilibrium open systems.
在光激发的体半导体中对激子的玻色-爱因斯坦凝聚(BEC)进行明确观测并阐明其内在性质,一直是凝聚态物理中的长期问题。在此,我们通过使用在稀释制冷机中实现的中红外诱导吸收成像直接在实空间中可视化激子云,观测到了低于400 mK的体CuO中1s仲激子捕获气体中出现的量子相变和玻色-爱因斯坦凝聚。我们的研究表明,传统的发光光谱无法检测到仲激子凝聚。我们发现凝聚分数异常小,仅为0.016,凝聚体的空间分布可用平均场理论很好地描述。我们在与冷声子浴相互作用的纯类物质激子系统中发现这种新型BEC,可能为其长程序的分类以及对非平衡开放系统量子统计力学的基本理解铺平道路。