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通过抑制界面缺陷发射增强在超薄GaAs缓冲层/Si模板上生长的1.3μm InAs量子点的光致发光

Enhanced Photoluminescence of 1.3 μm InAs Quantum Dots Grown on Ultrathin GaAs Buffer/Si Templates by Suppressing Interfacial Defect Emission.

作者信息

Kim Yeonhwa, Chu Rafael Jumar, Ryu Geunhwan, Woo Seungwan, Lung Quang Nhat Dang, Ahn Dae-Hwan, Han Jae-Hoon, Choi Won Jun, Jung Daehwan

机构信息

Center for Opto-electronic Materials and Devices, Korea Institute of Science and Technology, Seoul 02792, South Korea.

Division of Nano & Information Technology, University of Science and Technology, Seoul 02792, South Korea.

出版信息

ACS Appl Mater Interfaces. 2022 Oct 5;14(39):45051-45058. doi: 10.1021/acsami.2c14492. Epub 2022 Sep 26.

Abstract

We report on the photoluminescence enhancement of 1.3 μm InAs quantum dots (QDs) epitaxially grown on an ultrathin 250 nm GaAs buffer on a Si substrate. Decreasing the GaAs buffer thickness from 1000 to 250 nm was found to not only increase the coalesced QD density from 6.5 × 10 to 1.9 × 10 cm but also decrease the QD photoluminescence emission intensity dramatically. Inserting an AlGaAs potential barrier layer maintained strong photoluminescence from the QDs by effectively suppressing carrier leakage to the GaAs/Si interfacial region even when the GaAs buffer was thinned to 250 nm. We then fabricated a light-emitting diode using the ultrathin 250 nm GaAs buffer on Si and confirmed strong electroluminescence peaking at 1.28 μm without interfacial defect emission at room temperature. We believe that this work is promising for monolithically integrated evanescent Si lasers using InAs/GaAs QDs.

摘要

我们报道了在硅衬底上超薄250纳米砷化镓缓冲层上外延生长的1.3微米砷化铟量子点的光致发光增强情况。发现将砷化镓缓冲层厚度从1000纳米减小到250纳米,不仅会使合并量子点密度从6.5×10增加到1.9×10厘米,还会显著降低量子点的光致发光发射强度。插入一个铝镓砷势垒层,即使将砷化镓缓冲层减薄到250纳米,也能通过有效抑制载流子泄漏到砷化镓/硅界面区域,从而保持量子点的强光致发光。然后,我们使用硅上超薄250纳米砷化镓缓冲层制作了一个发光二极管,并证实其在室温下有强电致发光,峰值在1.28微米,且无界面缺陷发射。我们认为这项工作对于使用砷化铟/砷化镓量子点的单片集成倏逝硅激光器很有前景。

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