Xu Longmeng, Niu Haoyu, Bai Yuming, Zhu Haipeng, Yuan Songliu, He Xiong, Han Yibo, Zhao Lingxiao, Yang Yang, Xia Zhengcai, Liang Qifeng, Tian Zhaoming
Wuhan National High Magnetic Field Center, Huazhong University of Science and Technology, Wuhan 430074, People's Republic of China.
School of Physics, Huazhong University of Science and Technology, Wuhan 430074, People's Republic of China.
J Phys Condens Matter. 2022 Oct 18;34(48). doi: 10.1088/1361-648X/ac987a.
The RAlX (R = Light rare earth; X = Ge, Si) compounds, as a family of magnetic Weyl semimetal, have recently attracted growing attention due to the tunability of Weyl nodes and its interactions with diverse magnetism by rare-earth atoms. Here, we report the magnetotransport evidence and electronic structure calculations on nontrivial band topology of SmAlSi, a new member of this family. At low temperatures, SmAlSi exhibits large non-saturated magnetoresistance (MR) (as large as ∼5500% at 2 K and 48 T) and distinct Shubnikov-de Haas (SdH) oscillations. The field dependent MRs at 2 K deviate from the semiclassical ()variation but follow the power-law relation MR∝()with a crossover from∼ 1.52 at low fields (< 15 T) to∼ 1 under high fields (> 18 T), which is attributed to the existence of Weyl points and electron-hole compensated characteristics with high mobility. From the analysis of SdH oscillations, two fundamental frequencies originating from the Fermi surface pockets with non-trivialBerry phases and small cyclotron mass can be identified, this feature is supported by the calculated electronic band structures with two Weyl pockets near the Fermi level. Our study establishes SmAlSi as a paradigm for researching the novel topological states of RAlX family.
作为磁性外尔半金属家族的一员,RAlX(R = 轻稀土;X = 锗、硅)化合物最近因其外尔节点的可调性以及稀土原子与多种磁性的相互作用而受到越来越多的关注。在此,我们报告了该家族新成员SmAlSi非平凡能带拓扑的磁输运证据和电子结构计算。在低温下,SmAlSi表现出大的非饱和磁电阻(MR)(在2 K和48 T时高达约5500%)以及明显的舒布尼科夫 - 德哈斯(SdH)振荡。2 K时的场依赖磁电阻偏离半经典()变化,但遵循幂律关系MR∝(),在低场(< 15 T)时从约1.52交叉到高场(> 18 T)时的约1,这归因于外尔点的存在以及具有高迁移率的电子 - 空穴补偿特性。通过对SdH振荡的分析,可以识别出源于具有非平凡贝里相位和小回旋质量的费米面口袋的两个基本频率,这一特征得到了在费米能级附近有两个外尔口袋计算电子能带结构的支持。我们的研究将SmAlSi确立为研究RAlX家族新型拓扑态的范例。