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巨磁电阻材料中手性轨道电流的控制。

Control of chiral orbital currents in a colossal magnetoresistance material.

机构信息

Department of Physics, University of Colorado at Boulder, Boulder, CO, USA.

School of Physics, Georgia Institute of Technology, Atlanta, GA, USA.

出版信息

Nature. 2022 Nov;611(7936):467-472. doi: 10.1038/s41586-022-05262-3. Epub 2022 Oct 12.

Abstract

Colossal magnetoresistance (CMR) is an extraordinary enhancement of the electrical conductivity in the presence of a magnetic field. It is conventionally associated with a field-induced spin polarization that drastically reduces spin scattering and electric resistance. Ferrimagnetic MnSiTe is an intriguing exception to this rule: it exhibits a seven-order-of-magnitude reduction in ab plane resistivity that occurs only when a magnetic polarization is avoided. Here, we report an exotic quantum state that is driven by ab plane chiral orbital currents (COC) flowing along edges of MnTe octahedra. The c axis orbital moments of ab plane COC couple to the ferrimagnetic Mn spins to drastically increase the ab plane conductivity (CMR) when an external magnetic field is aligned along the magnetic hard c axis. Consequently, COC-driven CMR is highly susceptible to small direct currents exceeding a critical threshold, and can induce a time-dependent, bistable switching that mimics a first-order 'melting transition' that is a hallmark of the COC state. The demonstrated current-control of COC-enabled CMR offers a new paradigm for quantum technologies.

摘要

巨磁电阻(CMR)是指在磁场存在的情况下电导率的非凡增强。它通常与磁场诱导的自旋极化有关,这种极化极大地减少了自旋散射和电阻。亚铁磁 MnSiTe 是这一规则的一个有趣例外:当避免磁场极化时,它在 ab 平面的电阻率会降低七个数量级。在这里,我们报告了一种奇特的量子态,它是由沿 MnTe 八面体边缘流动的 ab 平面手性轨道电流(COC)驱动的。当外磁场沿磁硬 c 轴对齐时,ab 平面 COC 的 c 轴轨道矩与亚铁磁 Mn 自旋耦合,极大地增加了 ab 平面的电导率(CMR)。因此,COC 驱动的 CMR 对超过临界阈值的小直流电流非常敏感,并可以诱导类似于 COC 状态标志的一阶“熔化转变”的时变双稳态切换。所展示的 COC 实现的 CMR 的电流控制为量子技术提供了一个新的范例。

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