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石墨烯热载流子快速通道实现的强增强太赫兹波产生

Strongly enhanced THz generation enabled by a graphene hot-carrier fast lane.

作者信息

Zhang Dehui, Xu Zhen, Cheng Gong, Liu Zhe, Gutierrez Audrey Rose, Zang Wenzhe, Norris Theodore B, Zhong Zhaohui

机构信息

Department of Electrical Engineering and Computer Science, University of Michigan, Ann Arbor, MI, 48109, USA.

出版信息

Nat Commun. 2022 Oct 27;13(1):6404. doi: 10.1038/s41467-022-34170-3.

Abstract

Semiconductor photoconductive switches are useful and versatile emitters of terahertz (THz) radiation with a broad range of applications in THz imaging and time-domain spectroscopy. One fundamental challenge for achieving efficient ultrafast switching, however, is the relatively long carrier lifetime in most common semiconductors. To obtain picosecond ultrafast pulses, especially when coupled with waveguides/transmission lines, semiconductors are typically engineered with high defect density to reduce the carrier lifetimes, which in turn lowers the overall power output of the photoconductive switches. To overcome this fundamental trade-off, here we present a new hybrid photoconductive switch design by engineering a hot-carrier fast lane using graphene on silicon. While photoexcited carriers are generated in the silicon layer, similar to a conventional switch, the hot carriers are transferred to the graphene layer for efficient collection at the contacts. As a result, the graphene-silicon hybrid photoconductive switch emits THz fields with up to 80 times amplitude enhancement compared to its graphene-free counterpart. These results both further the understanding of ultrafast hot carrier transport in such hybrid systems and lay the groundwork toward intrinsically more powerful THz devices based on 2D-3D hybrid heterostructures.

摘要

半导体光电导开关是有用且通用的太赫兹(THz)辐射源,在太赫兹成像和时域光谱学中有广泛应用。然而,实现高效超快开关的一个基本挑战是大多数常见半导体中相对较长的载流子寿命。为了获得皮秒级超快脉冲,特别是当与波导/传输线耦合时,半导体通常设计有高缺陷密度以降低载流子寿命,这反过来又降低了光电导开关的整体功率输出。为了克服这种基本的权衡,我们在此提出一种新的混合光电导开关设计,通过在硅上使用石墨烯设计一条热载流子快速通道。与传统开关类似,虽然光激发载流子在硅层中产生,但热载流子被转移到石墨烯层以便在接触点处有效收集。结果,与无石墨烯的同类开关相比,石墨烯 - 硅混合光电导开关发射的太赫兹场的幅度增强了高达80倍。这些结果既进一步加深了对这种混合系统中超快热载流子传输的理解,也为基于二维 - 三维混合异质结构的本质上更强大的太赫兹器件奠定了基础。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/ad7d/9613981/a85a1c46f160/41467_2022_34170_Fig1_HTML.jpg

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