Chatterjee Sudipta, Sau Jyotirmay, Ghosh Subrata, Samanta Saheli, Ghosh Barnali, Kumar Manoranjan, Mandal Kalyan
S. N. Bose National Centre for Basic Sciences, Block JD, Sector III, Salt Lake, Kolkata 700106, India.
J Phys Condens Matter. 2022 Nov 16;51(3). doi: 10.1088/1361-648X/aca0d7.
Magnetic topological semimetals (TSMs) with broken time-reversal symmetry are very rare and have drawn significant attention in condensed matter physics due to their numerous intriguing topological properties. Among these various magnetic TSMs, Co-based full Heusler compounds are of current interest, since a few of these materials exhibit Weyl and nodal fermions in their topological band structure. In this work, we report a comprehensive study of anomalous Hall effect (AHE) in the ferromagnetic full Heusler compound CoVAl. Recent studies indicate that the intrinsic AHE is closely related to the Berry curvature of the occupied electronic Bloch states. The present study of CoVAl attempts to understand and explore the possibility of topology-induced AHE. The anomalous Hall resistivityρxyAis observed to scale quadratically with the longitudinal resistivity. Our experimental results also reveal that the anomalous Hall conductivity (AHC) is ∼85 cmat 2 K with an intrinsic contribution of ∼75.6 S cm, and is nearly insensitive to temperature. The first principle calculations note that the Berry curvature originated from a gapped nodal line and symmetry-protected Weyl nodes near the Fermi level (EF) is the main source of AHE in this compound. Thus, this investigation on CoVAl discloses that it is a ferromagnetic Weyl and nodal-line TSM. The theoretically calculated AHC is in well agreement with the experimentally obtained AHC.
具有时间反演对称性破缺的磁性拓扑半金属(TSMs)非常罕见,因其众多有趣的拓扑性质而在凝聚态物理领域引起了广泛关注。在这些各种各样的磁性TSMs中,基于钴的全赫斯勒化合物目前备受关注,因为其中一些材料在其拓扑能带结构中表现出外尔费米子和节线费米子。在这项工作中,我们报告了对铁磁全赫斯勒化合物CoVAl中反常霍尔效应(AHE)的全面研究。最近的研究表明,本征AHE与占据的电子布洛赫态的贝里曲率密切相关。对CoVAl的当前研究试图理解和探索拓扑诱导AHE的可能性。观察到反常霍尔电阻率ρxyA与纵向电阻率呈二次方比例关系。我们的实验结果还表明,反常霍尔电导率(AHC)在2 K时约为85 S/cm,本征贡献约为75.6 S/cm,并且几乎对温度不敏感。第一性原理计算表明,源于带隙节线和费米能级(EF)附近对称保护的外尔节点的贝里曲率是该化合物中AHE的主要来源。因此,对CoVAl的这项研究表明它是一种铁磁外尔和节线TSM。理论计算的AHC与实验获得的AHC非常吻合。