Department of Physics, Stockholm University, 106 91 Stockholm, Sweden.
Max Born Institute for Nonlinear Optics and Short Pulse Spectroscopy, 12489 Berlin, Germany.
J Synchrotron Radiat. 2022 Nov 1;29(Pt 6):1454-1464. doi: 10.1107/S1600577522008414. Epub 2022 Sep 29.
The advent of X-ray free-electron lasers (XFELs) has revolutionized fundamental science, from atomic to condensed matter physics, from chemistry to biology, giving researchers access to X-rays with unprecedented brightness, coherence and pulse duration. All XFEL facilities built until recently provided X-ray pulses at a relatively low repetition rate, with limited data statistics. Here, results from the first megahertz-repetition-rate X-ray scattering experiments at the Spectroscopy and Coherent Scattering (SCS) instrument of the European XFEL are presented. The experimental capabilities that the SCS instrument offers, resulting from the operation at megahertz repetition rates and the availability of the novel DSSC 2D imaging detector, are illustrated. Time-resolved magnetic X-ray scattering and holographic imaging experiments in solid state samples were chosen as representative, providing an ideal test-bed for operation at megahertz rates. Our results are relevant and applicable to any other non-destructive XFEL experiments in the soft X-ray range.
X 射线自由电子激光(XFEL)的出现彻底改变了基础科学,从原子到凝聚态物理,从化学到生物学,为研究人员提供了前所未有的亮度、相干性和脉冲持续时间的 X 射线。直到最近,所有建造的 XFEL 设施都以相对较低的重复率提供 X 射线脉冲,数据统计有限。本文介绍了在欧洲 XFEL 的光谱学和相干散射(SCS)仪器上进行的首次兆赫兹重复率 X 射线散射实验的结果。本文说明了 SCS 仪器在兆赫兹重复率下运行以及新型 DSSC 2D 成像探测器的可用性所带来的实验能力。选择固态样品的时间分辨磁 X 射线散射和全息成像实验作为代表性实验,为在兆赫兹速率下运行提供了理想的测试平台。我们的结果与软 X 射线范围内的任何其他非破坏性 XFEL 实验相关且适用。