Iacocca E, Liu T-M, Reid A H, Fu Z, Ruta S, Granitzka P W, Jal E, Bonetti S, Gray A X, Graves C E, Kukreja R, Chen Z, Higley D J, Chase T, Le Guyader L, Hirsch K, Ohldag H, Schlotter W F, Dakovski G L, Coslovich G, Hoffmann M C, Carron S, Tsukamoto A, Kirilyuk A, Kimel A V, Rasing Th, Stöhr J, Evans R F L, Ostler T, Chantrell R W, Hoefer M A, Silva T J, Dürr H A
Department of Applied Mathematics, University of Colorado, Boulder, CO, 80309, USA.
National Institute of Standards and Technology, Boulder, CO, 80305, USA.
Nat Commun. 2019 Apr 15;10(1):1756. doi: 10.1038/s41467-019-09577-0.
Sub-picosecond magnetisation manipulation via femtosecond optical pumping has attracted wide attention ever since its original discovery in 1996. However, the spatial evolution of the magnetisation is not yet well understood, in part due to the difficulty in experimentally probing such rapid dynamics. Here, we find evidence of a universal rapid magnetic order recovery in ferrimagnets with perpendicular magnetic anisotropy via nonlinear magnon processes. We identify magnon localisation and coalescence processes, whereby localised magnetic textures nucleate and subsequently interact and grow in accordance with a power law formalism. A hydrodynamic representation of the numerical simulations indicates that the appearance of noncollinear magnetisation via optical pumping establishes exchange-mediated spin currents with an equivalent 100% spin polarised charge current density of 10 A cm. Such large spin currents precipitate rapid recovery of magnetic order after optical pumping. The magnon processes discussed here provide new insights for the stabilization of desired meta-stable states.
自1996年首次发现以来,通过飞秒光泵浦进行亚皮秒级磁化操控一直备受关注。然而,磁化的空间演化尚未得到很好的理解,部分原因在于实验探测这种快速动力学存在困难。在此,我们通过非线性磁振子过程发现了具有垂直磁各向异性的亚铁磁体中普遍存在快速磁序恢复的证据。我们识别出磁振子局域化和合并过程,即局域磁结构成核,随后按照幂律形式相互作用并生长。数值模拟的流体动力学表示表明,通过光泵浦产生的非共线磁化的出现建立了交换介导的自旋电流,其等效的100%自旋极化电荷电流密度为10 A/cm。如此大的自旋电流促使光泵浦后磁序快速恢复。这里讨论的磁振子过程为所需亚稳态的稳定提供了新的见解。