Institute for Integrative Nanosciences (IIN), Leibniz Institute for Solid State and Materials Research (IFW) Dresden, Helmholtzstraße 20, D-01069, Dresden, Germany.
Universidad Autónoma del Estado de Morelos, Ave. Universidad 1001, CP, 62209, Cuernavaca, Morelos, México.
Sci Rep. 2023 Jan 6;13(1):292. doi: 10.1038/s41598-023-27404-x.
Transition metal dichalcogenide (TMD) semiconductors are two-dimensional materials with great potential for the future of nano-optics and nano-optoelectronics as well as the rich and exciting development of basic research. The influence of an external magnetic field on a TMD monolayer raises a new question: to unveil the behavior of the magneto-polaron resonances (MPRs) associated with the phonon symmetry inherent in the system. It is shown that the renormalized Landau energy levels are modified by the interplay of the long-range Pekar-Fröhlich (PF) and short-range deformation potential (DP) interactions. This leads to a new series of MPRs involving the optical phonons at the center of the Brillouin zone. The coupling of the two Landau levels with the LO and [Formula: see text] optical phonon modes provokes resonant splittings of double avoided-crossing levels giving rise to three excitation branches. This effect appears as bigger energy gaps at the anticrossing points in the renormalized Landau levels. To explore the interplay between the MPRs, the electron-phonon interactions (PF and DP) and the couplings between adjacent Landau levels, a full Green's function treatment for the evaluation of the energy and its life-time broadening is developed. A generalization of the two-level approach is performed for the description of the new MPR branches. The obtained results are a guideline for the magneto-optical experiments in TMDs, where three MPR peaks should be observable.
过渡金属二卤族化合物(TMD)半导体是二维材料,具有在纳米光学和纳米光电子学方面的巨大潜力,同时也为基础研究的丰富和令人兴奋的发展提供了可能。外磁场对 TMD 单层的影响提出了一个新的问题:揭示与系统固有声子对称性相关的磁极化子共振(MPR)的行为。结果表明,长程 Pekar-Fröhlich(PF)和短程变形势(DP)相互作用会改变重整化的朗道能级。这导致了一系列新的 MPR,涉及到布里渊区中心的光学声子。两个朗道能级与 LO 和 [Formula: see text] 光学声子模式的耦合引起了双避免交叉能级的共振分裂,从而产生了三个激发分支。这种效应表现为在重整化的朗道能级的交叉点处出现更大的能隙。为了探索 MPR、电子-声子相互作用(PF 和 DP)以及相邻朗道能级之间的耦合之间的相互作用,开发了一种全格林函数方法来评估能量及其寿命展宽。对两能级方法进行了推广,以描述新的 MPR 分支。所得结果为 TMD 中的磁光实验提供了指导,在该实验中应该可以观察到三个 MPR 峰。