Zhang Liyang, Guo Yuntao, Tie Jinfeng, Yao Zenghui, Feng Zihao, Wu Qiong, Wang Xinxin, Luo Haiyun
Department of Electrical Engineering, Tsinghua University, Beijing 100084, China.
Department of Electrical Engineering, Tsinghua University, Beijing 100084, China.
J Hazard Mater. 2023 Apr 5;447:130780. doi: 10.1016/j.jhazmat.2023.130780. Epub 2023 Jan 13.
Atmospheric pressure dielectric barrier discharge (DBD) plasma is an emerging technique for effective bioaerosol decontamination and is promising to be used in indoor environments to reduce infections. However, fundamental knowledge of the dose and dose-response characteristics of plasma-based disinfection technology is very limited. By examining the single-pass removal efficiency of S. lentus aerosol by in-duct grating-like DBD plasma reactors with varied discharge setups (gap distance, electrode size, number of discharge layers, frequency, dielectric material), it was found that the specific input energy (SIE) could be served as the dose for disinfection, and the efficiency was exponentially dependent on SIE in most cases. The corresponding susceptibility constants (Z values) were obtained hereinafter. Humidity was a prominent factor boosting the efficiency with a Z value of 0.36 L/J at relative humidity (RH) of 20% and 1.68 L/J at RH of 60%. MS2 phage showed a much higher efficiency of 2.66-3.08 log of reduction than those of S. lentus (38-85%) and E. coli (42%-95%) under the same condition. Using SIE as the dose, the performance of plasma reactors in the literature was compared and evaluated. This work provides a theoretical and engineering basis for air disinfection by plasma-based technology.
大气压介质阻挡放电(DBD)等离子体是一种用于有效生物气溶胶去污的新兴技术,有望用于室内环境以减少感染。然而,基于等离子体的消毒技术的剂量和剂量响应特性的基础知识非常有限。通过研究具有不同放电设置(间隙距离、电极尺寸、放电层数、频率、介电材料)的管道内格栅状DBD等离子体反应器对迟缓芽孢杆菌气溶胶的单次去除效率,发现比输入能量(SIE)可作为消毒剂量,并且在大多数情况下效率与SIE呈指数关系。随后获得了相应的敏感性常数(Z值)。湿度是提高效率的一个显著因素,在相对湿度(RH)为20%时Z值为0.36 L/J,在RH为60%时Z值为1.68 L/J。在相同条件下,MS2噬菌体的去除效率比迟缓芽孢杆菌(38%-85%)和大肠杆菌(42%-95%)高得多,可达2.66-3.08个对数级的减少。以SIE作为剂量,对文献中报道的等离子体反应器性能进行了比较和评估。这项工作为基于等离子体技术的空气消毒提供了理论和工程基础。