Interdisciplinary Materials Research Center, Institute for Advanced Study, Chengdu University, Chengdu, 610106, P. R. China.
School of Chemistry and Chemical Engineering, Yangzhou University, Yangzhou, Jiangsu, 225009, P. R. China.
Adv Sci (Weinh). 2023 Apr;10(10):e2206887. doi: 10.1002/advs.202206887. Epub 2023 Jan 22.
The use of metal-organic frameworks (MOFs) in solid-state electrolytes (SSEs) has been a very attractive research area that has received widespread attention in the modern world. SSEs can be divided into different types, some of which can be combined with MOFs to improve the electrochemical performance of the batteries by taking advantage of the high surface area and high porosity of MOFs. However, it also faces many serious problems and challenges. In this review, different types of SSEs are classified and the changes in these electrolytes after the addition of MOFs are described. Afterward, these SSEs with MOFs attached are introduced for different types of battery applications and the effects of these SSEs combined with MOFs on the electrochemical performance of the cells are described. Finally, some challenges faced by MOFs materials in batteries applications are presented, then some solutions to the problems and development expectations of MOFs are given.
金属-有机骨架（MOFs）在固态电解质（SSEs）中的应用是一个非常有吸引力的研究领域，在现代社会受到了广泛关注。SSEs 可以分为不同的类型，其中一些可以与 MOFs 结合，利用 MOFs 的高比表面积和高孔隙率来提高电池的电化学性能。然而，它也面临着许多严重的问题和挑战。在这篇综述中，对不同类型的 SSEs 进行了分类，并描述了 MOFs 加入后这些电解质的变化。随后，介绍了这些与 MOFs 结合的 SSEs 在不同类型电池中的应用，以及这些 SSEs 与 MOFs 结合对电池电化学性能的影响。最后，提出了 MOFs 材料在电池应用中面临的一些挑战，然后给出了一些解决问题的方法和对 MOFs 发展的期望。
