EaStCHEM School of Chemistry, Biomedical Sciences Research Complex, and Centre of Magnetic Resonance, University of St Andrews, North Haugh, St AndrewsKY16 9ST, U.K.
Department of Chemistry, University of Copenhagen, CopenhagenDK-2100, Denmark.
J Am Chem Soc. 2023 Feb 8;145(5):2877-2883. doi: 10.1021/jacs.2c10902. Epub 2023 Jan 25.
We demonstrate by use of continuous wave- and pulse-electron paramagnetic resonance spectroscopy on oriented single crystals of magnetically dilute Yb ions in YbLu(trensal) that molecular entangled two-qubit systems can be constructed by exploiting dipolar interactions between neighboring Yb centers. Furthermore, we show that the phase memory time and Rabi frequencies of these dipolar-interaction-coupled entangled two-qubit systems are comparable to the ones of the corresponding single qubits.
我们通过使用连续波和脉冲电子顺磁共振光谱技术,在 YbLu(trensal) 中磁性稀释 Yb 离子的取向单晶上进行了演示,证明了可以通过利用相邻 Yb 中心之间的偶极相互作用来构建分子纠缠双量子比特系统。此外,我们还表明,这些偶极相互作用耦合的纠缠双量子比特系统的相位记忆时间和拉比频率与相应的单量子比特相当。