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中国中部典型工业化地区土壤重金属污染风险的时空格局及增量驱动力

Spatiotemporal patterns of soil heavy metal pollution risk and driving forces of increment in a typical industrialized region in central China.

作者信息

Yang Xue, Yang Yong

机构信息

College of Resources and Environment, Huazhong Agricultural University, Wuhan 430070, China.

Key Laboratory of Arable Land Conservation (Middle and Lower Reaches of the Yangtze River), Ministry of Agriculture, China.

出版信息

Environ Sci Process Impacts. 2023 Mar 22;25(3):554-565. doi: 10.1039/d2em00487a.

Abstract

Excessive enrichment of soil heavy metals seriously damages human health and soil environment. Exploring the spatiotemporal patterns and detecting the influencing factors are conducive to developing targeted risk management and control. Based on the soil samples of Co, Cr, Cu, Mn, Ni, Pb, Zn, and Cd collected in one typical industrialized region in China from 2016 to 2019, this study analyzed the spatiotemporal pattern of geo-accumulation risk and potential ecological risk based on the spatiotemporal ordinary kriging (STOK) prediction, and probed the driving forces of heavy metal increments with the random forest (RF) regression model. The risk assessment revealed that soils were seriously contaminated by Pb, Cd, and Cu, moderately contaminated by Zn and Mn, and uncontaminated by Co, Cr, and Ni; more than 30% of areas had moderate to high potential ecological risks. From 2016 to 2019, soil heavy metal contents increased in more than 50% of regions and the growth rates of accumulations were ranked as Co (65%) > Ni (56%) > Mn (43%) > Pb (40%) > Cr (36%) > Zn (31%) > Cu (23%) > Cd (3%). High contents and increases of heavy metals in soils near industrial lands are higher. Smelter (24%), mine (20%), and factory (12%) were the major contributing factors for these heavy metal increments, followed by transportation (6%) and population (5%). The results indicated that the management of industrial discharge and contaminated soils should be strengthened to prevent the worsening soil heavy metal pollution in the study area.

摘要

土壤重金属过度富集严重损害人类健康和土壤环境。探索其时空格局并检测影响因素有助于制定针对性的风险管理与控制措施。基于2016年至2019年在中国一个典型工业化地区采集的钴、铬、铜、锰、镍、铅、锌和镉的土壤样本,本研究基于时空普通克里格(STOK)预测分析了地累积风险和潜在生态风险的时空格局,并利用随机森林(RF)回归模型探究了重金属增量的驱动力。风险评估显示,土壤受到铅、镉和铜的严重污染,锌和锰的中度污染,钴、铬和镍未受污染;超过30%的区域具有中度至高潜在生态风险。2016年至2019年,超过50%的区域土壤重金属含量增加,累积增长率排序为钴(65%)>镍(56%)>锰(43%)>铅(40%)>铬(36%)>锌(31%)>铜(23%)>镉(3%)。工业用地附近土壤中重金属的高含量和增加幅度更高。冶炼厂(24%)、矿山(20%)和工厂(12%)是这些重金属增量的主要贡献因素,其次是交通(6%)和人口(5%)。结果表明,应加强工业排放和污染土壤的管理,以防止研究区域土壤重金属污染恶化。

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