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通过阳极电镀和热煅烧可扩展合成BiVO薄膜。

Scalable synthesis of BiVO thin films via anodic plating and thermal calcination.

作者信息

Jiang Haoyang, Xiao Yongcheng, Zhong Miao

机构信息

College of Engineering and Applied Sciences, Nanjing University, 163 Xianlin Avenue, Qixia District, Nanjing, 210023, China.

出版信息

Discov Nano. 2023 Feb 8;18(1):6. doi: 10.1186/s11671-023-03774-z.

DOI:10.1186/s11671-023-03774-z
PMID:36752997
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC9908786/
Abstract

Fabrication of high-quality semiconductor thin films has long been a subject of keen interest in the photocatalytic field. Here, we report a facile, solution-based anodic plating and calcination for large-scale synthesis of BiVO thin films on indium tin oxide coated glass for use as photoanodes in solar water splitting. Using NaSO as a sacrificial reagent, continuous solar H production with 94% Faradaic efficiency was obtained over 6 h of photoelectrochemical water splitting.

摘要

长期以来，高质量半导体薄膜的制备一直是光催化领域备受关注的课题。在此，我们报道了一种简便的、基于溶液的阳极电镀和煅烧方法，用于在氧化铟锡涂层玻璃上大规模合成BiVO薄膜，用作太阳能水分解中的光阳极。使用NaSO作为牺牲试剂，在光电化学水分解6小时的过程中，实现了法拉第效率为94%的连续太阳能制氢。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/aff2/9908786/ca76be59c6e8/11671_2023_3774_Fig5_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/aff2/9908786/c3a9c4ff7b79/11671_2023_3774_Fig1_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/aff2/9908786/e537b1da15cc/11671_2023_3774_Fig2_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/aff2/9908786/8714ca71dcaa/11671_2023_3774_Fig3_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/aff2/9908786/7236ddb6d48a/11671_2023_3774_Fig4_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/aff2/9908786/ca76be59c6e8/11671_2023_3774_Fig5_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/aff2/9908786/c3a9c4ff7b79/11671_2023_3774_Fig1_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/aff2/9908786/e537b1da15cc/11671_2023_3774_Fig2_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/aff2/9908786/8714ca71dcaa/11671_2023_3774_Fig3_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/aff2/9908786/7236ddb6d48a/11671_2023_3774_Fig4_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/aff2/9908786/ca76be59c6e8/11671_2023_3774_Fig5_HTML.jpg

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本文引用的文献

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Long-term solar water and CO splitting with photoelectrochemical BiOI-BiVO tandems.利用光电化学BiOI-BiVO串联电池进行长期太阳能水分解和二氧化碳分解
Nat Mater. 2022 Aug;21(8):864-868. doi: 10.1038/s41563-022-01262-w. Epub 2022 May 26.
2
Stable, active CO reduction to formate via redox-modulated stabilization of active sites.通过氧化还原调节活性位点的稳定性，实现稳定、高效的一氧化碳还原为甲酸盐。
Nat Commun. 2021 Sep 1;12(1):5223. doi: 10.1038/s41467-021-25573-9.
3
Accelerated discovery of CO electrocatalysts using active machine learning.使用主动机器学习加速 CO 电催化剂的发现。
Nature. 2020 May;581(7807):178-183. doi: 10.1038/s41586-020-2242-8. Epub 2020 May 13.
4
Photoelectrochemical devices for solar water splitting - materials and challenges.用于太阳能水分解的光电化学器件-材料与挑战。
Chem Soc Rev. 2017 Jul 31;46(15):4645-4660. doi: 10.1039/c6cs00306k.
5
Surface Modification of CoO(x) Loaded BiVO₄ Photoanodes with Ultrathin p-Type NiO Layers for Improved Solar Water Oxidation.CoO(x) 负载的 BiVO₄ 光阳极的超薄 p 型 NiO 层表面修饰用于提高太阳能水氧化。
J Am Chem Soc. 2015 Apr 22;137(15):5053-60. doi: 10.1021/jacs.5b00256. Epub 2015 Apr 9.
6
Nanoporous BiVO4 photoanodes with dual-layer oxygen evolution catalysts for solar water splitting.具有双层析氧催化剂的介孔 BiVO4 光阳极用于太阳能水分解。
Science. 2014 Feb 28;343(6174):990-4. doi: 10.1126/science.1246913. Epub 2014 Feb 13.
7
Efficient solar water splitting by enhanced charge separation in a bismuth vanadate-silicon tandem photoelectrode.在铋钒酸盐-硅串联光电极中通过增强电荷分离实现高效太阳能水分解。
Nat Commun. 2013;4:2195. doi: 10.1038/ncomms3195.
8
Efficient and stable photo-oxidation of water by a bismuth vanadate photoanode coupled with an iron oxyhydroxide oxygen evolution catalyst.铋钒酸盐光阳极与铁氧体羟基氧化物析氧催化剂协同作用促进水的高效稳定光氧化。
J Am Chem Soc. 2012 Feb 1;134(4):2186-92. doi: 10.1021/ja209001d. Epub 2012 Jan 20.
9
Wireless solar water splitting using silicon-based semiconductors and earth-abundant catalysts.基于硅基半导体和丰富的地球催化剂的无线太阳能水分解。
Science. 2011 Nov 4;334(6056):645-8. doi: 10.1126/science.1209816. Epub 2011 Sep 29.
10
Photoelectrochemical cells.光电化学电池
Nature. 2001 Nov 15;414(6861):338-44. doi: 10.1038/35104607.