Zhang Ruo Peng, Mei Mei, Qiu Huihe
Department of Mechanical and Aerospace Engineering, The Hong Kong University of Science & Technology, Clear Water Bay, Kowloon 999077, Hong Kong SAR, China.
Thrust of Sustainable Energy and Environment, The Hong Kong University of Science and Technology (Guangzhou), Guangzhou 511453, China.
Langmuir. 2023 Feb 28;39(8):3083-3093. doi: 10.1021/acs.langmuir.2c03175. Epub 2023 Feb 20.
Roughness on hydrophilic surfaces allows for fast propagation of liquids. In this paper, the hypothesis is tested which theorizes that pillar array structures with nonuniform pillar height levels can enhance wicking rates. In this work, within a unit cell, nonuniform micropillars were arranged with one pillar at constant height, while other shorter pillars were varied in height to study these nonuniform effects. Subsequently, a new microfabrication technique was developed to fabricate a nonuniform pillar array surface. Capillary rising-rate experiments were conducted with water, decane, and ethylene glycol as working liquids to determine the behavior of propagation coefficients that were dependent on pillar morphology. It is found that a nonuniform pillar height structure leads to a separation of layers in the liquid spreading process and the propagation coefficient increases with declining micropillar height for all liquids tested. This indicated a significant enhancement of wicking rates compared to uniform pillar arrays. A theoretical model was subsequently developed to explain and predict the enhancement effect by considering capillary force and viscous resistance of nonuniform pillar structures. The insights and implications from this model thus advance our understanding of the physics of the wicking process and can inform the design of pillar structures with an enhanced wicking propagation coefficient.
亲水性表面的粗糙度有利于液体的快速传播。在本文中,对一个假设进行了验证,该假设理论认为具有不均匀柱高的柱状阵列结构可以提高芯吸速率。在这项工作中,在一个单元胞内,将不均匀的微柱排列成一个柱高恒定,而其他较短的柱高则变化,以研究这些不均匀效应。随后,开发了一种新的微制造技术来制造不均匀的柱状阵列表面。以水、癸烷和乙二醇作为工作液体进行了毛细管上升速率实验,以确定取决于柱形态的传播系数的行为。研究发现,不均匀的柱高结构在液体铺展过程中会导致分层,并且对于所有测试液体,传播系数随微柱高度的降低而增加。这表明与均匀柱状阵列相比,芯吸速率有显著提高。随后建立了一个理论模型,通过考虑不均匀柱结构的毛细力和粘性阻力来解释和预测增强效果。该模型的见解和意义因此推进了我们对芯吸过程物理原理的理解,并可为具有增强芯吸传播系数的柱结构设计提供参考。