Department of Physics, Harvard University, Cambridge, MA 02138.
Department of Physics, Massachusetts Institute of Technology, Cambridge, MA 02139.
Proc Natl Acad Sci U S A. 2023 Feb 28;120(9):e2219208120. doi: 10.1073/pnas.2219208120. Epub 2023 Feb 24.
The quantization of the electromagnetic field leads directly to the existence of quantum mechanical states, called Fock states, with an exact integer number of photons. Despite these fundamental states being long-understood, and despite their many potential applications, generating them is largely an open problem. For example, at optical frequencies, it is challenging to deterministically generate Fock states of order two and beyond. Here, we predict the existence of an effect in nonlinear optics, which enables the deterministic generation of large Fock states at arbitrary frequencies. The effect, which we call an -photon bound state in the continuum, is one in which a photonic resonance (such as a cavity mode) becomes lossless when a precise number of photons is inside the resonance. Based on analytical theory and numerical simulations, we show that these bound states enable a remarkable phenomenon in which a coherent state of light, when injected into a system supporting this bound state, can spontaneously evolve into a Fock state of a controllable photon number. This effect is also directly applicable for creating (highly) squeezed states of light, whose photon number fluctuations are (far) below the value expected from classical physics (i.e., shot noise). We suggest several examples of systems to experimentally realize the effects predicted here in nonlinear nanophotonic systems, showing examples of generating both optical Fock states with large ( > 10), as well as more macroscopic photonic states with very large squeezing, with over 90% less noise (10 dB) than the classical value associated with shot noise.
电磁场的量子化直接导致了量子力学态的存在,这些态被称为福克态(Fock states),其光子数为精确的整数。尽管这些基本态已经被长期理解,并且尽管它们有许多潜在的应用,但它们的产生在很大程度上仍是一个开放的问题。例如,在光学频率下,很难确定性地产生阶数为二及更高的福克态。在这里,我们预测了一种非线性光学中的效应的存在,该效应可以在任意频率下确定性地产生大的福克态。该效应,我们称之为连续谱中的 -光子束缚态,是指当精确数量的光子处于共振中时,光子共振(如腔模)变得无损耗。基于解析理论和数值模拟,我们表明这些束缚态使相干光态在注入支持这种束缚态的系统时,可以自发演化成可控光子数的福克态,这一现象非常显著。该效应也可直接用于产生(高)压缩态的光,其光子数的涨落远低于经典物理预期的值(即,散粒噪声)。我们提出了几种非线性纳米光子系统中实验实现所预测的效应的系统示例,展示了产生具有大光子数(>10)的光学福克态的例子,以及具有非常大压缩的更宏观的光子态,其噪声比与散粒噪声相关的经典值低 10 分贝(10 dB)以上。