Rivera Nicholas
School of Applied and Engineering Physics, Cornell University, Ithaca, NY 14853, USA.
Department of Physics, Harvard University, Cambridge, MA 02139, USA.
Nanophotonics. 2025 Mar 31;14(11):1837-1855. doi: 10.1515/nanoph-2024-0605. eCollection 2025 Jun.
Nonlinear dynamics provide an indispensable resource for creating quantum states of light, as well as other bosonic systems. Seminal work using second- and third-order nonlinear optical crystals, cavity quantum electrodynamics, and superconducting circuits, have enabled generating squeezed states, as well as various non-Gaussian quantum states (e.g., single photons, cat states) at both infrared and microwave frequencies. Nevertheless, it remains challenging to generate quantum states of light in broad portions of the electromagnetic spectrum: for example, at terahertz frequencies and at ultraviolet and X-ray frequencies. In this Perspective, I discuss a variety of emerging material platforms, as well as emerging theoretical and experimental tools, which enable overcoming these challenges. The main argument of this Perspective is that advances in driving nonlinear dynamics of material excitations, will enable generating quantum states of these material excitations as well as quantum states of light at new frequency ranges. I will further argue that in order to realize much of the promise of this nascent field, there is a need for innovation in the laser systems used to drive these nonlinear dynamics: specifically, innovations in realizing high-power laser sources that have very low noise, having quantum statistics similar to coherent states of light which describe lower intensity laser systems. I will highlight some experimental and theoretical work, in understanding quantum noise dynamics in complex laser systems, that can address these challenges.
非线性动力学为创建光的量子态以及其他玻色子系统提供了不可或缺的资源。利用二阶和三阶非线性光学晶体、腔量子电动力学以及超导电路的开创性工作,已能够在红外和微波频率下生成压缩态以及各种非高斯量子态(例如单光子、猫态)。然而,在电磁频谱的大部分频段生成光的量子态仍然具有挑战性:例如,在太赫兹频率以及紫外和X射线频率下。在这篇观点文章中,我将讨论各种新兴的材料平台以及新兴的理论和实验工具,这些能够克服这些挑战。这篇观点文章的主要论点是,推动材料激发的非线性动力学方面的进展,将能够在新的频率范围内生成这些材料激发的量子态以及光的量子态。我还将进一步指出,为了实现这个新兴领域的诸多前景,需要在用于驱动这些非线性动力学的激光系统方面进行创新:具体而言,要在实现具有极低噪声的高功率激光源方面进行创新,使其具有类似于描述低强度激光系统的光的相干态的量子统计特性。我将重点介绍一些在理解复杂激光系统中的量子噪声动力学方面的实验和理论工作,这些工作能够应对这些挑战。