Liu Yan, Tian Yun, Xu Jianda, Wang Changfu, Wang Yun, Yuan Dingzhong, Chew Jia Wei
Engineering Research Center of Nuclear Technology Application (East China Institute of Technology), Ministry of Education Nanchang 330013 China
School of Chemical and Biomedical Engineering, Nanyang Technological University Singapore 637459 Singapore
RSC Adv. 2023 Feb 24;13(10):6518-6529. doi: 10.1039/d2ra08252g. eCollection 2023 Feb 21.
Due to its unique advantages such as flexible planar structure, ultrahigh specific surface area, superior electrical conductivity and electrical double-layer capacitance in theory, graphene has unparalleled virtues compared with other carbon materials. This review summarizes the recent research progress of various graphene-based electrodes on ion electrosorption fields, especially for water desalination utilizing capacitive deionization (CDI) technology. We present the latest advances of graphene-based electrodes, such as 3D graphene, graphene/metal oxide (MO) composites, graphene/carbon composites, heteroatom-doped graphene and graphene/polymer composites. Furthermore, a brief outlook on the challenges and future possible developments in the electrosorption area are also addressed for researchers to design graphene-based electrodes towards practical application.
由于石墨烯具有独特的优势,如平面结构灵活、比表面积超高、导电性优异以及理论上具有双电层电容,与其他碳材料相比,它具有无与伦比的优点。本文综述了各种基于石墨烯的电极在离子电吸附领域的最新研究进展,特别是利用电容去离子化(CDI)技术进行水脱盐方面的进展。我们介绍了基于石墨烯的电极的最新进展,如三维石墨烯、石墨烯/金属氧化物(MO)复合材料、石墨烯/碳复合材料、杂原子掺杂石墨烯和石墨烯/聚合物复合材料。此外,还简要展望了电吸附领域的挑战和未来可能的发展方向,以供研究人员设计基于石墨烯的电极以实现实际应用。