School of Materials Science and Engineering, Beihang University, Beijing, 100191, China.
State Key Laboratory of Metastable Materials Science and Technology, Yanshan University, Qinhuangdao, 066004, China.
Adv Sci (Weinh). 2023 May;10(13):e2300193. doi: 10.1002/advs.202300193. Epub 2023 Mar 8.
Many functional materials are approaching their performance limits due to inherent trade-offs between essential physical properties. Such trade-offs can be overcome by engineering a material that has an ordered arrangement of structural units, including constituent components/phases, grains, and domains. By rationally manipulating the ordering with abundant structural units at multiple length scales, the structural ordering opens up unprecedented opportunities to create transformative functional materials, as amplified properties or disruptive functionalities can be realized. In this perspective article, a brief overview of recent advances in the emerging ordered functional materials across catalytic, thermoelectric, and magnetic materials regarding the fabrication, structure, and property is presented. Then the possibility of applying this structural ordering strategy to highly efficient neuromorphic computing devices and durable battery materials is discussed. Finally, remaining scientific challenges are highlighted, and the prospects for ordered functional materials are made. This perspective aims to draw the attention of the scientific community to the emerging ordered functional materials and trigger intense studies on this topic.
由于基本物理性质之间存在固有的权衡,许多功能材料的性能已接近其极限。通过工程设计具有结构单元有序排列的材料,可以克服这种权衡,这些结构单元包括组成成分/相、晶粒和畴。通过在多个长度尺度上合理地操纵丰富的结构单元的有序性,结构有序性为创造变革性功能材料提供了前所未有的机会,因为可以实现放大的性能或颠覆性的功能。在这篇观点文章中,简要综述了在催化、热电和磁性材料方面新兴有序功能材料在制造、结构和性能方面的最新进展。然后讨论了将这种结构有序策略应用于高效神经形态计算器件和耐用电池材料的可能性。最后,突出了存在的科学挑战,并对有序功能材料的前景进行了展望。本观点旨在引起科学界对新兴有序功能材料的关注,并引发对此主题的深入研究。