Nanolithography and Application Research Group, School of Information Science and Technology, Fudan University, Shanghai 200433, People's Republic of China.
Shanghai Synchrotron Radiation Facility, Shanghai Advanced Research Institute, Chinese Academy of Sciences, Shanghai 201210, People's Republic of China.
J Synchrotron Radiat. 2023 Mar 1;30(Pt 2):319-326. doi: 10.1107/S1600577522012115. Epub 2023 Feb 17.
With fast advances in enhancing the focusing/imaging resolution of Fresnel zone plate lenses toward sub-10 nm, low diffraction efficiency in connection with their rectangular zone shape still remains a big issue in both soft and hard X-ray microscopy. In hard X-ray optics, encouraging progress has recently been reported in our earlier attempts of high focusing efficiency by 3D kinoform shaped metallic zone plates, formed by greyscale electron beam lithography. This paper addresses our efforts towards high focusing/imaging efficiency by developing a novel dielectric kinoform zone plate lens for soft X-rays. The effects of the zone materials and zone shapes on the focusing/imaging quality were first theoretically investigated by a modified thin-grating-approximation method, revealing superior efficiencies of dielectric kinoform zone plates over rectangular ones in metals. Optical characterizations of replicated dielectric kinoform zone plates by greyscale electron beam lithography demonstrate a focusing efficiency of 15.5% with a resolution of 110 nm in the water window of X-rays. Apart from high efficiency, the novel kinoform zone plate lenses developed in this work exhibit significant advantages over conventional zone plates, i.e. simplified process, low cost and no need for a beamstop.
随着菲涅尔波带片透镜聚焦/成像分辨率向亚 10nm 迈进,其矩形波带形状导致的低衍射效率仍然是软 X 射线和硬 X 射线显微镜领域的一个大问题。在硬 X 射线光学中,我们早前通过灰阶电子束光刻形成的三维正弦形金属波带片实现了高聚焦效率,这方面取得了令人鼓舞的进展。本文通过开发用于软 X 射线的新型介电波带片透镜,致力于实现高聚焦/成像效率。通过改进的薄光栅近似法,首先从理论上研究了波带材料和波带形状对聚焦/成像质量的影响,结果表明介电波带片的效率优于金属中的矩形波带片。采用灰阶电子束光刻复制介电波带片的光学特性表明,在 X 射线水窗中,其聚焦效率为 15.5%,分辨率为 110nm。除了高效率,本文开发的新型正弦形波带片透镜与传统波带片相比还具有显著优势,即工艺简化、成本低且无需光阑。