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高效构建可持续细菌纤维素气凝胶,通过调整功能基团提高 PM 过滤效率。

Highly efficient construction of sustainable bacterial cellulose aerogels with boosting PM filter efficiency by tuning functional group.

机构信息

Institute of Chemicobiology and Functional Materials, School of Chemistry and Chemical Engineering, Nanjing University of Science and Technology, Nanjing 210094, China.

Institute of Chemicobiology and Functional Materials, School of Chemistry and Chemical Engineering, Nanjing University of Science and Technology, Nanjing 210094, China.

出版信息

Carbohydr Polym. 2023 Jun 1;309:120664. doi: 10.1016/j.carbpol.2023.120664. Epub 2023 Feb 9.

Abstract

Air pollution has become a major public health concern, attracting considerable attention from researchers working on environmentally friendly and sustainable materials. In this work, bacterial cellulose (BC) derived aerogels were fabricated by the directional ice-templated method and used as filters to remove PM particles. We modified the surface functional groups of BC aerogel with reactive silane precursors, and investigated the interfacial and structural properties of those aerogels. The results show that BC-derived aerogels have excellent compressive elasticity, and their directional growth orientation inside the structure significantly reduced pressure drop. Moreover, the BC-derived filters exhibit an exceptional quantitative removal effect on fine particulate matter, which, in the presence of high concentrations of fine particulate matter, they can achieve a high-efficiency removal standard of 95 %. Meanwhile, the BC-derived aerogels showed superior biodegradation performance in the soil burial test. These results paved the way for BC-derived aerogels development as a great sustainable alternative to treat air pollution.

摘要

空气污染已成为主要的公共卫生关注点,吸引了从事环保和可持续材料研究的人员的极大关注。在这项工作中,采用定向冰模板法制备了细菌纤维素(BC)衍生气凝胶,并将其用作过滤材料以去除 PM 颗粒。我们用反应性硅烷前体对 BC 气凝胶的表面官能团进行了改性,并研究了这些气凝胶的界面和结构性能。结果表明,BC 衍生气凝胶具有优异的压缩弹性,其结构内部的定向生长取向显著降低了压降。此外,BC 衍生的过滤器对细颗粒物具有出色的定量去除效果,在细颗粒物浓度较高的情况下,它们可以达到 95%的高效去除标准。同时,BC 衍生气凝胶在土壤掩埋试验中表现出优异的生物降解性能。这些结果为开发 BC 衍生气凝胶作为一种处理空气污染的可持续替代品铺平了道路。

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