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纳米粒子的随机平均磁中子散射截面的各向异性。

On the angular anisotropy of the randomly averaged magnetic neutron scattering cross section of nanoparticles.

机构信息

Department of Physics and Materials Science, University of Luxembourg, 162A avenue de la Faiencerie, L-1511 Luxembourg, Grand Duchy of Luxembourg.

出版信息

IUCrJ. 2023 May 1;10(Pt 3):261-269. doi: 10.1107/S205225252300180X.

DOI:10.1107/S205225252300180X
PMID:36913314
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC10161771/
Abstract

The magnetic small-angle neutron scattering (SANS) cross section of dilute ensembles of uniformly magnetized and randomly oriented Stoner-Wohlfarth particles is calculated using the Landau-Lifshitz equation. The focus of this study is on the angular anisotropy of the magnetic SANS signal as it can be seen on a two-dimensional position-sensitive detector. Depending on the symmetry of the magnetic anisotropy of the particles (e.g. uniaxial, cubic), an anisotropic magnetic SANS pattern may result, even in the remanent state or at the coercive field. The case of inhomogeneously magnetized particles and the effects of a particle-size distribution and interparticle correlations are also discussed.

摘要

使用朗道-利夫希茨方程计算了均匀磁化且随机取向的斯通纳-沃尔夫哈特粒子稀集会的磁小角中子散射(SANS)截面。本研究的重点是磁 SANS 信号的各向异性,因为它可以在二维位置灵敏探测器上看到。根据粒子磁各向异性的对称性(例如单轴、立方),即使在剩磁状态或矫顽场下,也可能会出现各向异性的磁 SANS 模式。本文还讨论了不均匀磁化粒子的情况以及粒径分布和粒子间相关性的影响。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/97c0/10161771/d7f127dba13b/m-10-00261-fig5.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/97c0/10161771/266eaef3c363/m-10-00261-fig1.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/97c0/10161771/1a8ae2a7f839/m-10-00261-fig2.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/97c0/10161771/fc4127c565e4/m-10-00261-fig3.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/97c0/10161771/ca2c295b470b/m-10-00261-fig4.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/97c0/10161771/d7f127dba13b/m-10-00261-fig5.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/97c0/10161771/266eaef3c363/m-10-00261-fig1.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/97c0/10161771/1a8ae2a7f839/m-10-00261-fig2.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/97c0/10161771/fc4127c565e4/m-10-00261-fig3.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/97c0/10161771/ca2c295b470b/m-10-00261-fig4.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/97c0/10161771/d7f127dba13b/m-10-00261-fig5.jpg

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本文引用的文献

1
Magnetic neutron scattering from spherical nanoparticles with Néel surface anisotropy: analytical treatment.具有奈尔表面各向异性的球形纳米颗粒的磁中子散射:解析处理
J Appl Crystallogr. 2022 Nov 4;55(Pt 6):1475-1487. doi: 10.1107/S1600576722008925. eCollection 2022 Dec 1.
2
Magnetic neutron scattering from spherical nanoparticles with Néel surface anisotropy: atomistic simulations.具有奈尔表面各向异性的球形纳米颗粒的磁中子散射:原子模拟
J Appl Crystallogr. 2022 Nov 4;55(Pt 6):1488-1499. doi: 10.1107/S1600576722008949. eCollection 2022 Dec 1.
3
Using small-angle scattering to guide functional magnetic nanoparticle design.
利用小角散射指导功能性磁性纳米颗粒的设计。
Nanoscale Adv. 2022 Jan 17;4(4):1026-1059. doi: 10.1039/d1na00482d. eCollection 2022 Feb 15.
4
Signature of antiphase boundaries in iron oxide nanoparticles.氧化铁纳米颗粒中反相边界的特征
J Appl Crystallogr. 2021 Nov 16;54(Pt 6):1719-1729. doi: 10.1107/S1600576721010128. eCollection 2021 Dec 1.
5
Embracing Defects and Disorder in Magnetic Nanoparticles.拥抱磁性纳米粒子中的缺陷与无序。
Adv Sci (Weinh). 2021 Feb 15;8(7):2002682. doi: 10.1002/advs.202002682. eCollection 2021 Apr.
6
Origin of reduced magnetization and domain formation in small magnetite nanoparticles.小磁铁矿纳米颗粒中磁化强度降低和畴形成的起源。
Sci Rep. 2017 Apr 10;7:45997. doi: 10.1038/srep45997.
7
Anisotropy of the structure factor of magnetic fluids under a field probed by small-angle neutron scattering.磁场作用下磁流体结构因子的各向异性:小角中子散射探测
Phys Rev E Stat Nonlin Soft Matter Phys. 2002 Mar;65(3 Pt 1):031403. doi: 10.1103/PhysRevE.65.031403. Epub 2002 Feb 15.