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不同排放情景下北京未来新粒子形成的预估。

Estimates of Future New Particle Formation under Different Emission Scenarios in Beijing.

机构信息

School of Geography, Earth & Environmental Sciences University of Birmingham, Birmingham B15 2TT, United Kingdom.

Department of Environmental Sciences, Faculty of Meteorology, Environment and Arid Land Agriculture, King Abdulaziz University, Jeddah 21589, Saudi Arabia.

出版信息

Environ Sci Technol. 2023 Mar 28;57(12):4741-4750. doi: 10.1021/acs.est.2c08348. Epub 2023 Mar 17.

Abstract

New particle formation (NPF) is a leading source of particulate matter by number and a contributor to particle mass during haze events. Reductions in emissions of air pollutants, many of which are NPF precursors, are expected in the move toward carbon neutrality or net-zero. Expected changes to pollutant emissions are used to investigate future changes to NPF processes, in comparison to a simulation of current conditions. The projected changes to SO emissions are key in changing future NPF number, with different scenarios producing either a doubling or near total reduction in sulfuric acid-amine particle formation rates. Particle growth rates are projected to change little in all but the strictest emission control scenarios. These changes will reduce the particle mass arising by NPF substantially, thus showing a further cobenefit of net-zero policies. Major uncertainties remain in future NPF including the volatility of oxygenated organic molecules resulting from changes to NO and amine emissions.

摘要

新粒子形成(NPF)是数量最多的颗粒物的主要来源,也是霾事件期间颗粒物质量的主要贡献者。在向碳中和或净零排放过渡的过程中,预计会减少空气污染物的排放,其中许多都是 NPF 的前体。预计污染物排放的变化将用于研究与当前条件模拟相比,NPF 过程的未来变化。SO 排放的预计变化是改变未来 NPF 数量的关键,不同的情景会导致硫酸-胺粒子形成速率翻倍或几乎完全减少。除了最严格的排放控制情景外,预计所有情景的颗粒生长速率变化都很小。这些变化将大大减少由 NPF 引起的颗粒质量,从而表明净零政策的进一步协同效益。未来的 NPF 仍存在重大不确定性,包括由于 NO 和胺排放的变化而导致的含氧有机分子的挥发性。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a488/10061929/09f65cbbf5b4/es2c08348_0001.jpg

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