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介质粘弹性对相互作用的多分散气泡泡内塌缩强度的影响

Effects of medium viscoelasticity on bubble collapse strength of interacting polydisperse bubbles.

作者信息

Qin Dui, Zou Qingqin, Zhong Xianhua, Zhang Bingyu, Li Zhangyong

机构信息

Department of Biomedical Engineering, School of Bioinformatics, Chongqing University of Posts and Telecommunications, Chongqing, People's Republic of China; Postdoctoral Workstation of Chongqing People's Hospital, Chongqing, People's Republic of China.

Department of Biomedical Engineering, School of Bioinformatics, Chongqing University of Posts and Telecommunications, Chongqing, People's Republic of China.

出版信息

Ultrason Sonochem. 2023 May;95:106375. doi: 10.1016/j.ultsonch.2023.106375. Epub 2023 Mar 17.

Abstract

Due to its physical and/or chemical effects, acoustic cavitation plays a crucial role in various emerging applications ranging from advanced materials to biomedicine. The cavitation bubbles usually undergo oscillatory dynamics and violent collapse within a viscoelastic medium, which are closely related to the cavitation-associated effects. However, the role of medium viscoelasticity on the cavitation dynamics has received little attention, especially for the bubble collapse strength during multi-bubble cavitation with the complex interactions between size polydisperse bubbles. In this study, modified Gilmore equations accounting for inter-bubble interactions were coupled with the Zener viscoelastic model to simulate the dynamics of multi-bubble cavitation in viscoelastic media. Results showed that the cavitation dynamics (e.g., acoustic resonant response, nonlinear oscillation behavior and bubble collapse strength) of differently-sized bubbles depend differently on the medium viscoelasticity and each bubble is affected by its neighboring bubbles to a different degree. More specifically, increasing medium viscosity drastically dampens the bubble dynamics and weakens the bubble collapse strength, while medium elasticity mainly affects the bubble resonance at which the bubble collapse strength is maximum. Differently-sized bubbles can achieve resonances and even subharmonic resonances at high driving acoustic pressures as the elasticity changes to certain values, and the resonance frequency of each bubble increases with the elasticity increasing. For the interactions between the size polydisperse bubbles, it indicated that the largest bubble generally has a dominant effect on the dynamics of smaller ones while in turn it is almost unaffected, exhibiting a pattern of destructive and constructive interactions. This study provides a valuable insight into the acoustic cavitation dynamics of multiple interacting polydisperse bubbles in viscoelastic media, which may offer a potential of controlling the medium viscoelasticity to appropriately manipulate the dynamics of multi-bubble cavitation for achieving proper cavitation effects according to the desired application.

摘要

由于其物理和/或化学效应,声空化在从先进材料到生物医学等各种新兴应用中发挥着关键作用。空化气泡通常在粘弹性介质中经历振荡动力学和剧烈坍塌,这与空化相关效应密切相关。然而,介质粘弹性对空化动力学的作用很少受到关注,特别是对于多泡空化过程中气泡坍塌强度,其中大小多分散气泡之间存在复杂的相互作用。在本研究中,考虑气泡间相互作用的修正吉尔摩方程与齐纳粘弹性模型相结合,以模拟粘弹性介质中多泡空化的动力学。结果表明,不同大小气泡的空化动力学(如声共振响应、非线性振荡行为和气泡坍塌强度)对介质粘弹性的依赖程度不同,每个气泡受到其相邻气泡的影响程度也不同。更具体地说,增加介质粘度会极大地抑制气泡动力学并削弱气泡坍塌强度,而介质弹性主要影响气泡坍塌强度最大时的气泡共振。随着弹性变化到一定值,不同大小的气泡在高驱动声压下可以实现共振甚至亚谐波共振,并且每个气泡的共振频率随着弹性增加而增加。对于大小多分散气泡之间的相互作用,表明最大的气泡通常对较小气泡的动力学具有主导作用,而反过来它几乎不受影响,呈现出破坏性和建设性相互作用的模式。本研究为粘弹性介质中多个相互作用的多分散气泡的声空化动力学提供了有价值的见解,这可能提供控制介质粘弹性以适当操纵多泡空化动力学的潜力,从而根据期望的应用实现适当的空化效果。

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