Li Ding, Lu Qing, Cai Limei, Chen Laiguo, Wang Hanzhi
Hubei Key Laboratory of Petroleum Geochemistry and Environment, Yangtze University, Wuhan 430100, China.
Key Laboratory of Exploration Technologies for Oil and Gas Resources, Ministry of Education, Yangtze University, Wuhan 430100, China.
Toxics. 2023 Mar 10;11(3):257. doi: 10.3390/toxics11030257.
In this study, we compared the concentrations of the heavy metals Cd, Cr, Cu, Zn, Ni, and Pb in the surface soils of urban parks in Wuhan, Hubei Province, with those in the surface soils of urban parks worldwide. The soil contamination data were assessed using enrichment factors and spatial analysis of heavy metals using inverse distance weighting and quantitative analysis of heavy metal sources with a positive definite matrix factor (PMF) receptor model. Further, a probabilistic health risk assessment of children and adults using Monte Carlo simulation was performed. The average Cd, Cr, Cu, Zn, Ni, and Pb concentrations in the surface soils of urban parks were 2.52, 58.74, 31.39, 186.28, 27.00, and 34.89 mg·kg, respectively, which exceeded the average soil background values in Hubei. From the inverse distance spatial interpolation map, heavy metal contamination was primarily observed to be present to the southwest of the main urban area. The PMF model resolved four sources: mixed traffic and industrial emission, natural, agricultural, and traffic sources, with relative contributions of 23.9%, 19.3%, 23.4%, and 33.4%, respectively. The Monte Carlo health risk evaluation model demonstrated negligible noncancer risks for both adult and child populations, whereas the health effects of Cd and Cr on children were a concern for cancer risks.
在本研究中,我们比较了湖北省武汉市城市公园表层土壤中重金属镉(Cd)、铬(Cr)、铜(Cu)、锌(Zn)、镍(Ni)和铅(Pb)的浓度与全球城市公园表层土壤中的浓度。使用富集因子评估土壤污染数据,采用反距离加权法对重金属进行空间分析,并使用正定矩阵因子(PMF)受体模型对重金属来源进行定量分析。此外,还使用蒙特卡洛模拟对儿童和成人进行了概率健康风险评估。城市公园表层土壤中Cd、Cr、Cu、Zn、Ni和Pb的平均浓度分别为2.52、58.74、31.39、186.28、27.00和34.89 mg·kg,均超过了湖北土壤背景值的平均水平。从反距离空间插值图可以看出,重金属污染主要集中在主城区的西南部。PMF模型解析出四个来源:混合交通和工业排放源、自然源、农业源和交通源,其相对贡献率分别为23.9%、19.3%、23.4%和33.4%。蒙特卡洛健康风险评估模型表明,成人和儿童人群的非致癌风险可忽略不计,而Cd和Cr对儿童的健康影响则是癌症风险方面的一个关注点。