Key Laboratory of Soil Environment and Pollution Remediation, Institute of Soil Science, Chinese Academy of Sciences, Nanjing 210008, China.
Key Laboratory of Soil Environment and Pollution Remediation, Institute of Soil Science, Chinese Academy of Sciences, Nanjing 210008, China; University of Chinese Academy of Sciences, Beijing 100049, China.
Sci Total Environ. 2021 Aug 1;780:146557. doi: 10.1016/j.scitotenv.2021.146557. Epub 2021 Mar 18.
Identification and quantification of the distribution, ecological risk, and sources of heavy metals in soils are essential for regional pollution control and management. In this study, spatial analysis (SA), GeogDetector model (GDM), and positive matrix factorization (PMF) model were combined to evaluate the status, ecological risk, and sources of heavy metals in soils from a typical coastal economic development area in Southeastern China. The mean contents of Cd, Pb, Cr, Cu, and Zn in the surface soils (0-20 cm) were 0.45, 41.72, 90.50, 47.86, and 145.33 mg/kg, respectively. In accordance, the mean contents of Cd exceeded the risk screening value for contamination of agricultural soil in China. Our results revealed that industrial and residential soils had higher enrichment of heavy metals than agricultural and fallow soils. Industrial production was the major driving factors influencing the spatial distribution of heavy metals. Soil OM and pH were found to be the most important factors affecting the potential ecological risk of heavy metals, followed by distance from the industrial enterprises and roads. Heavy metals in the study area were mainly originated from industrial emissions/atmospheric deposition, agricultural sources, and followed by natural sources. Therefore, regular monitoring and source control for heavy metals, especially for Cd, along with the integrated soil environmental management in the study area are crucial to ensure soil health and ecosystem security.
识别和量化土壤中重金属的分布、生态风险和来源,对于区域污染控制和管理至关重要。本研究采用空间分析(SA)、地理探测器模型(GDM)和正定矩阵因子分解(PMF)模型相结合的方法,评估了中国东南部一个典型沿海经济发展区土壤中重金属的现状、生态风险和来源。表层土壤(0-20cm)中 Cd、Pb、Cr、Cu 和 Zn 的平均含量分别为 0.45、41.72、90.50、47.86 和 145.33mg/kg。相应地,Cd 的平均含量超过了中国农业土壤污染风险筛选值。结果表明,工业和住宅土壤中重金属的富集程度高于农业和休耕地土壤。工业生产是影响重金属空间分布的主要驱动因素。土壤有机质和 pH 值是影响重金属潜在生态风险的最重要因素,其次是距工业企业和道路的距离。研究区的重金属主要来源于工业排放/大气沉降、农业源,其次是自然源。因此,定期监测和控制重金属,特别是 Cd,以及综合土壤环境管理,对于确保土壤健康和生态系统安全至关重要。