Lin Xiaohui, Yang Ruqi, Zhang Wen, Zeng Ning, Zhao Yu, Wang Guocheng, Li Tingting, Cai Qixiang
State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing, China.
State Key Laboratory of Numerical Modeling for Atmospheric Sciences and Geophysical Fluid Dynamics, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing, China.
Carbon Balance Manag. 2023 May 19;18(1):9. doi: 10.1186/s13021-023-00229-x.
Air pollution in China has raised great concerns due to its adverse effects on air quality, human health, and climate. Emissions of air pollutants (APs) are inherently linked with CO emissions through fossil-energy consumption. Knowledge of the characteristics of APs and CO emissions and their relationships is fundamentally important in the pursuit of co-benefits in addressing air quality and climate issues in China. However, the linkages and interactions between APs and CO in China are not well understood.
Here, we conducted an ensemble study of six bottom-up inventories to identify the underlying drivers of APs and CO emissions growth and to explore their linkages in China. The results showed that, during 1980-2015, the power and industry sectors contributed 61-79% to China's overall emissions of CO, NO, and SO. In addition, the residential and industrial sectors were large emitters (77-85%) of PM, PM, CO, BC, and OC. The emissions of CH, NO and NH were dominated by the agriculture sector (46-82%) during 1980-2015, while the share of CH emissions in the energy sector increased since 2010. During 1980-2015, APs and greenhouse gases (GHGs) emissions from residential sources generally decreased over time, while the transportation sector increased its impact on recent emissions, particularly for NO and NMVOC. Since implementation of stringent pollution control measures and accompanying technological improvements in 2013, China has effectively limited pollution emissions (e.g., growth rates of -10% per year for PM and -20% for SO) and slowed down the increasing trend of carbon emissions from the power and industrial sectors. We also found that areas with high emissions of CO, NO, NMVOC, and SO also emitted large amounts of CO, which demonstrates the possible common sources of APs and GHGs. Moreover, we found significant correlations between CO and APs (e.g., NO, CO, SO, and PM) emissions in the top 5% high-emitting grid cells, with more than 60% common grid cells during 2010-2015.
We found significant correlation in spatial and temporal aspects for CO, and NO, CO, SO, and PM emissions in China. We targeted sectorial and spatial APs and GHGs emission hot-spots, which help for management and policy-making of collaborative reductions of them. This comprehensive analysis over 6 datasets improves our understanding of APs and GHGs emissions in China during the period of rapid industrialization from 1980 to 2015. This study helps elucidate the linkages between APs and CO from an integrated perspective, and provides insights for future synergistic emissions reduction.
中国的空气污染因其对空气质量、人类健康和气候的不利影响而备受关注。空气污染物(APs)的排放与化石能源消耗产生的一氧化碳(CO)排放有着内在联系。了解空气污染物和一氧化碳排放的特征及其关系,对于在中国实现空气质量和气候问题协同效益的追求至关重要。然而,中国空气污染物和一氧化碳之间的联系与相互作用尚未得到充分理解。
在此,我们对六个自下而上的清单进行了综合研究,以确定空气污染物和一氧化碳排放增长的潜在驱动因素,并探索它们在中国的联系。结果表明,在1980 - 2015年期间,电力和工业部门对中国一氧化碳、氮氧化物(NO)和二氧化硫(SO)的总排放量贡献了61% - 79%。此外,居民和工业部门是细颗粒物(PM)、可吸入颗粒物(PM)、一氧化碳、黑碳(BC)和有机碳(OC)的大量排放源(77% - 85%)。在1980 - 2015年期间,甲烷(CH)、氮氧化物和氨(NH)的排放主要由农业部门主导(46% - 82%),而自2010年以来,能源部门甲烷排放的占比有所增加。在1980 - 2015年期间,居民源的空气污染物和温室气体(GHGs)排放总体上随时间减少,而交通运输部门对近期排放的影响增加,特别是氮氧化物和非甲烷挥发性有机物(NMVOC)。自2013年实施严格的污染控制措施并伴随技术改进以来,中国有效限制了污染排放(例如,细颗粒物每年-10%的增长率和二氧化硫-20%的增长率),并减缓了电力和工业部门碳排放的上升趋势。我们还发现,一氧化碳、氮氧化物、非甲烷挥发性有机物和二氧化硫高排放地区也排放大量的二氧化碳,这表明空气污染物和温室气体可能存在共同来源。此外,我们发现,在2010 - 2015年期间,前5%高排放网格单元中一氧化碳与空气污染物(如氮氧化物、一氧化碳、二氧化硫和细颗粒物)排放之间存在显著相关性,共同网格单元超过60%。
我们发现中国一氧化碳、氮氧化物、一氧化碳、二氧化硫和细颗粒物排放在空间和时间方面存在显著相关性。我们确定了部门和空间空气污染物及温室气体排放热点,这有助于对它们进行协同减排的管理和决策。对6个数据集的综合分析增进了我们对中国1980年至2015年快速工业化时期空气污染物和温室气体排放的理解。本研究有助于从综合角度阐明空气污染物和一氧化碳之间的联系,并为未来协同减排提供见解。