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用于同时去除细颗粒物和现场肉眼可读甲醛传感的高效双功能自组装电纺纳米纤维过滤器

Highly Efficient, Dual-Functional Self-Assembled Electrospun Nanofiber Filters for Simultaneous PM Removal and On-Site Eye-Readable Formaldehyde Sensing.

作者信息

Song Jin Yeong, Kim Seongmin, Park Jaeseong, Park Sang Min

机构信息

School of Mechanical Engineering, Pusan National University, 63-2 Busan University-Ro, Geumjeong-Gu, Busan, 46241 South Korea.

出版信息

Adv Fiber Mater. 2023;5(3):1088-1103. doi: 10.1007/s42765-023-00279-3. Epub 2023 Mar 9.

Abstract

UNLABELLED

Air pollution containing particulate matter (PM) and volatile organic compounds has caused magnificent burdens on individual health and global economy. Although advances in highly efficient or multifunctional nanofiber filters have been achieved, many existing filters can only deal with one type of air pollutant, such as capturing PM or absorbing and detecting toxic gas. Here, highly efficient, dual-functional, self-assembled electrospun nanofiber (SAEN) filters were developed for simultaneous PM removal and onsite eye-readable formaldehyde sensing fabricated on a commercial fabric mask. With the use of an electrolyte solution containing a formaldehyde-sensitive colorimetric agent as a collector during electrospinning, the one-step fabrication of the dual-functional SAEN filter on commercial masks, such as a fabric mask and a daily disposable mask, was achieved. The electrolyte solution also allowed the uniform deposition of electrospun nanofibers, thereby achieving the high efficiency of PM filtration with an increased quality factor up to twice that of commercial masks. The SAEN filter enabled onsite and eye-readable formaldehyde gas detection by changing its color from yellow to red under a 5 ppm concentrated formaldehyde gas atmosphere. The repetitive fabrication and detachment of the SAEN filter on a fabric mask minimized the waste of the mask while maintaining high filtration efficiency by replenishing the SAEN filters and reusing the fabric mask. Given the dual functionality of SAEN filters, this process could provide new insights into designing and developing high performance and dual-functional electrospun nanofiber filters for various applications, including individual protection and indoor purification applications.

SUPPLEMENTARY INFORMATION

The online version contains supplementary material available at 10.1007/s42765-023-00279-3.

摘要

未标注

含有颗粒物(PM)和挥发性有机化合物的空气污染给个人健康和全球经济带来了巨大负担。尽管在高效或多功能纳米纤维过滤器方面已取得进展,但许多现有过滤器只能处理一种类型的空气污染物,例如捕获PM或吸收和检测有毒气体。在此,开发了高效、双功能、自组装电纺纳米纤维(SAEN)过滤器,用于在商用织物口罩上同时去除PM和进行现场肉眼可读的甲醛传感。在静电纺丝过程中,使用含有对甲醛敏感的比色剂的电解质溶液作为收集器,实现了在商用口罩(如织物口罩和日常一次性口罩)上一步制备双功能SAEN过滤器。电解质溶液还使电纺纳米纤维均匀沉积,从而实现了PM过滤的高效率,质量因数提高到商用口罩的两倍。SAEN过滤器在5 ppm浓甲醛气体气氛下通过将颜色从黄色变为红色,实现了现场肉眼可读的甲醛气体检测。SAEN过滤器在织物口罩上的重复制备和拆卸,通过补充SAEN过滤器和重复使用织物口罩,最大限度地减少了口罩的浪费,同时保持了高过滤效率。鉴于SAEN过滤器的双重功能,该工艺可为设计和开发用于各种应用(包括个人防护和室内净化应用)的高性能双功能电纺纳米纤维过滤器提供新的见解。

补充信息

在线版本包含可在10.1007/s42765-023-00279-3获取的补充材料。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/7cd5/9996567/a87c227249a4/42765_2023_279_Fig1_HTML.jpg

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