Merkouri Loukia-Pantzechroula, Paksoy Aysun Ipek, Ramirez Reina Tomas, Duyar Melis S
School of Chemistry and Chemical Engineering, University of Surrey, Guildford GU2 7XH, United Kingdom.
Inorganic Chemistry Department and Materials Sciences Institute, University of Seville-CSIC, 41092 Seville, Spain.
ACS Catal. 2023 May 15;13(11):7230-7242. doi: 10.1021/acscatal.3c00880. eCollection 2023 Jun 2.
Since climate change keeps escalating, it is imperative that the increasing CO emissions be combated. Over recent years, research efforts have been aiming for the design and optimization of materials for CO capture and conversion to enable a circular economy. The uncertainties in the energy sector and the variations in supply and demand place an additional burden on the commercialization and implementation of these carbon capture and utilization technologies. Therefore, the scientific community needs to think out of the box if it is to find solutions to mitigate the effects of climate change. Flexible chemical synthesis can pave the way for tackling market uncertainties. The materials for flexible chemical synthesis function under a dynamic operation, and thus, they need to be studied as such. Dual-function materials are an emerging group of dynamic catalytic materials that integrate the CO capture and conversion steps. Hence, they can be used to allow some flexibility in the production of chemicals as a response to the changing energy sector. This Perspective highlights the necessity of flexible chemical synthesis by focusing on understanding the catalytic characteristics under a dynamic operation and by discussing the requirements for the optimization of materials at the nanoscale.
由于气候变化不断升级,对抗不断增加的一氧化碳排放势在必行。近年来,研究工作一直致力于设计和优化用于捕获和转化一氧化碳的材料,以实现循环经济。能源部门的不确定性以及供需变化给这些碳捕获和利用技术的商业化和实施带来了额外负担。因此,如果要找到缓解气候变化影响的解决方案,科学界需要跳出框框思考。灵活的化学合成可为应对市场不确定性铺平道路。用于灵活化学合成的材料在动态操作下发挥作用,因此需要以此种方式进行研究。双功能材料是一类新兴的动态催化材料,它整合了一氧化碳捕获和转化步骤。因此,它们可用于在化学品生产中提供一定的灵活性,以应对不断变化的能源部门。本视角通过专注于理解动态操作下的催化特性以及讨论纳米尺度材料优化的要求,强调了灵活化学合成的必要性。