Zhai Meixiang, Ye Jiejun, Jiang Yingqiao, Yuan Sujuan, Li Yuehua, Liu Yongguang, Dai Lei, Wang Ling, He Zhangxing
School of Chemical Engineering, North China University of Science and Technology, Tangshan 063009, Hebei, China.
School of Chemical Engineering, North China University of Science and Technology, Tangshan 063009, Hebei, China.
J Colloid Interface Sci. 2023 Dec;651:902-918. doi: 10.1016/j.jcis.2023.08.041. Epub 2023 Aug 7.
Biomass-derived carbon (BDC) materials are suitable as electrode or catalyst materials for vanadium redox flow battery (VRFB), owing to the characteristics of vast material sources, environmental friendliness, and multifarious structures. A timely and comprehensive review of the structure and property significantly facilitates the development of BDC materials. Here, the paper starts with the preparation of biomass materials, including carbonization and activation. It is designed to summarize the lastest developments in BDC materials of VRFB in four different structural dimensions from zero dimension (0D) to three dimension (3D). Every dimension begins with meticulously selected examples to introduce the structural characteristics of materials and then illustrates the improved performance of the VRFB due to the structure. Simultaneously, challenges, solutions, and prospects are indicated for the further development of BDC materials. Overall, this review will help researchers select excellent strategies for the fabrication of BDC materials, thereby facilitating the use of BDC materials in VRFB design.
生物质衍生碳（BDC）材料因其原料来源广泛、环境友好和结构多样的特点，适合用作钒氧化还原液流电池（VRFB）的电极或催化剂材料。及时全面地综述其结构与性能，将极大地推动BDC材料的发展。本文从生物质材料的制备入手，包括碳化和活化。旨在从零维（0D）到三维（3D）这四个不同结构维度总结VRFB中BDC材料的最新进展。每个维度都以精心挑选的实例开篇，介绍材料的结构特征，然后阐述由于该结构而使VRFB性能得到的提升。同时，针对BDC材料的进一步发展指出了挑战、解决方案和前景。总体而言，本综述将帮助研究人员选择制备BDC材料的优良策略，从而推动BDC材料在VRFB设计中的应用。
