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2013 - 2020年纽约州按城市化程度和社会人口统计学划分的超细颗粒物和细颗粒物的环境暴露差异

Environmental exposure disparities in ultrafine particles and PM by urbanicity and socio-demographics in New York state, 2013-2020.

作者信息

Nair Arshad Arjunan, Lin Shao, Luo Gan, Ryan Ian, Qi Quan, Deng Xinlei, Yu Fangqun

机构信息

Atmospheric Sciences Research Center, University at Albany, State University of New York, Albany, NY 12226, USA.

Department of Environmental Health Sciences, University at Albany, State University of New York, Rensselaer, NY 12144, USA; Department of Epidemiology and Biostatistics, University at Albany, State University of New York, Rensselaer, NY 12144, USA.

出版信息

Environ Res. 2023 Dec 15;239(Pt 2):117246. doi: 10.1016/j.envres.2023.117246. Epub 2023 Oct 6.

Abstract

BACKGROUND

The spatiotemporal and demographic disparities in exposure to ultrafine particles (UFP; number concentrations of particulate matter (PM) with diameter ≤0.1 μm), a key subcomponent of fine aerosols (PM; mass concentrations of PM ≤ 2.5 μm), have not been well studied.

OBJECTIVE

To quantify and compare the aerosol pollutant exposure disparities for UFP and PM by socio-demographic factors in New York State (NYS).

METHODS

Ambient atmospheric UFP and PM were quantified using a global three-dimensional model of chemical transport with state-of-the-science aerosol microphysical processes validated extensively with observations. We matched these to U.S. census demographic data for varied spatial scales (state, county, county subdivision) and derived population-weighted aerosol exposure estimates. Aerosol exposure disparities for each demographic and socioeconomic (SES) indicator, with a focus on race-ethnicity and income, were quantified for the period 2013-2020.

RESULTS

The average NYS resident was exposed to 4451 #·cm UFP and 7.87 μg·m PM in 2013-2020, but minority race-ethnicity groups were invariably exposed to greater daily aerosol pollution (UFP: +75.0% & PM: +16.2%). UFP has increased since 2017 and is temporally and seasonally out-of-phase with PM. Race-ethnicity exposure disparities for PM have declined over time; by -6% from 2013 to 2017 and plateaued thereafter despite its decreasing concentrations. In contrast, these disparities have increased (+12.5-13.5%) for UFP. The aerosol pollution exposure disparities were the highest for low-income minorities and were more amplified for UFP than PM DISCUSSION: We identified large disparities in aerosol pollution exposure by urbanization level and socio-demographics in NYS residents. Jurisdictions with higher proportions of race-ethnicity minorities, low-income residents, and greater urbanization were disproportionately exposed to higher concentrations of UFP and PM than other NYS residents. These race-ethnicity exposure disparities were much larger, more disproportionate, and unabating over time for UFP compared to PM across various income strata and levels of urbanicity.

摘要

背景

超细颗粒物(UFP;直径≤0.1μm的颗粒物数量浓度)是细气溶胶(PM;PM≤2.5μm的质量浓度)的关键子成分,其在时空和人口统计学方面的差异尚未得到充分研究。

目的

通过纽约州(NYS)的社会人口因素,量化和比较UFP和PM的气溶胶污染物暴露差异。

方法

使用全球三维化学传输模型对环境大气中的UFP和PM进行量化,该模型的气溶胶微物理过程已通过观测得到广泛验证。我们将这些数据与不同空间尺度(州、县、县分区)的美国人口普查人口数据进行匹配,并得出人口加权的气溶胶暴露估计值。对2013 - 2020年期间每个人口统计学和社会经济(SES)指标的气溶胶暴露差异进行了量化,重点关注种族和收入。

结果

2013 - 2020年期间,纽约州居民平均暴露于4451#·cm的UFP和7.87μg·m的PM,但少数种族群体始终暴露于更高的每日气溶胶污染(UFP:+75.0%,PM:+16.2%)。自2017年以来,UFP有所增加,并且在时间和季节上与PM不同步。PM的种族暴露差异随时间有所下降;从2013年到2017年下降了-6%,此后尽管浓度下降但趋于平稳。相比之下,UFP的这些差异有所增加(+12.5 - 13.5%)。低收入少数群体的气溶胶污染暴露差异最大,并且UFP的差异比PM更为明显。

讨论

我们发现纽约州居民在气溶胶污染暴露方面存在城市化水平和社会人口统计学方面的巨大差异。与其他纽约州居民相比,种族少数群体、低收入居民比例较高且城市化程度较高的司法管辖区不成比例地暴露于更高浓度的UFP和PM。在不同收入阶层和城市化水平上,与PM相比,UFP的这些种族暴露差异更大、更不成比例且随着时间推移没有减弱。

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