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1T-TaS 中腔介导的金属-绝缘体转变的热控制。

Cavity-mediated thermal control of metal-to-insulator transition in 1T-TaS.

机构信息

Department of Physics, Università degli Studi di Trieste, Trieste, Italy.

Elettra Sincrotrone Trieste, Trieste, Italy.

出版信息

Nature. 2023 Oct;622(7983):487-492. doi: 10.1038/s41586-023-06596-2. Epub 2023 Oct 18.

Abstract

Placing quantum materials into optical cavities provides a unique platform for controlling quantum cooperative properties of matter, by both weak and strong light-matter coupling. Here we report experimental evidence of reversible cavity control of a metal-to-insulator phase transition in a correlated solid-state material. We embed the charge density wave material 1T-TaS into cryogenic tunable terahertz cavities and show that a switch between conductive and insulating behaviours, associated with a large change in the sample temperature, is obtained by mechanically tuning the distance between the cavity mirrors and their alignment. The large thermal modification observed is indicative of a Purcell-like scenario in which the spectral profile of the cavity modifies the energy exchange between the material and the external electromagnetic field. Our findings provide opportunities for controlling the thermodynamics and macroscopic transport properties of quantum materials by engineering their electromagnetic environment.

摘要

将量子材料置于光学腔中,通过弱光和强光与物质的耦合,为控制物质的量子协同特性提供了一个独特的平台。在这里,我们报告了在相关固态材料中通过金属-绝缘体相变的实验证据,该实验证据来自于对光腔的可逆控制。我们将电荷密度波材料 1T-TaS 嵌入到低温可调太赫兹腔中,并表明通过机械调节腔镜之间的距离及其对准,可以在与样品温度发生较大变化相关的情况下,实现从导电到绝缘行为的切换。观察到的较大热修饰表明类似于普塞尔(Purcell)的情况,其中腔的光谱分布改变了材料与外部电磁场之间的能量交换。我们的发现为通过设计量子材料的电磁环境来控制其热力学和宏观输运性质提供了机会。

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