De Beule Christophe, Phong Võ Tiến, Mele E J
Department of Physics and Astronomy, University of Pennsylvania, Philadelphia, PA 19104.
Department of Physics and Materials Science, University of Luxembourg, Luxembourg L-1511, Luxembourg.
Proc Natl Acad Sci U S A. 2023 Oct 24;120(43):e2306384120. doi: 10.1073/pnas.2306384120. Epub 2023 Oct 19.
In two-dimensional artificial crystals with large real-space periodicity, the nonlinear current response to a large applied electric field can feature a strong angular dependence, which encodes information about the band dispersion and Berry curvature of isolated electronic Bloch minibands. Within the relaxation-time approximation, we obtain analytic expressions up to infinite order in the driving field for the current in a band-projected theory with time-reversal and trigonal symmetry. For a fixed field strength, the dependence of the current on the direction of the applied field is given by rose curves whose petal structure is symmetry constrained and is obtained from an expansion in real-space translation vectors. We illustrate our theory with calculations on periodically buckled graphene and twisted double bilayer graphene, wherein the discussed physics can be accessed at experimentally relevant field strengths.
在具有大实空间周期性的二维人工晶体中,对大外加电场的非线性电流响应可能具有强烈的角度依赖性,这编码了关于孤立电子布洛赫微带的能带色散和贝里曲率的信息。在弛豫时间近似下,我们在具有时间反演和三角对称性的能带投影理论中,得到了驱动场中直至无穷阶的电流解析表达式。对于固定的场强,电流对外加场方向的依赖性由玫瑰曲线给出,其花瓣结构受到对称性约束,并且是通过实空间平移矢量的展开得到的。我们通过对周期性褶皱石墨烯和扭曲双层双层石墨烯的计算来说明我们的理论,其中所讨论的物理现象可以在实验相关的场强下观察到。