Xu Hongwei, Liu Jingwei, Wei Sheng, Luo Jie, Gong Rui, Tian Siyuan, Yang Yiqi, Lei Yukun, Chen Xinman, Wang Jiahong, Zhong Gaokuo, Tang Yongbing, Wang Feng, Cheng Hui-Ming, Ding Baofu
Faculty of Materials Science and Engineering/Institute of Technology for Carbon Neutrality, Shenzhen Institute of Advanced Technology, Chinese Academy of Sciences, Shenzhen, Guangdong, 518055, China.
School of Semiconductor Science and Technology, South China Normal University, Foshan, Guangdong, 528225, China.
Light Sci Appl. 2023 Nov 22;12(1):278. doi: 10.1038/s41377-023-01327-8.
Low-dimensional materials exhibit unique quantum confinement effects and morphologies as a result of their nanoscale size in one or more dimensions, making them exhibit distinctive physical properties compared to bulk counterparts. Among all low-dimensional materials, due to their atomic level thickness, two-dimensional materials possess extremely large shape anisotropy and consequently are speculated to have large optically anisotropic absorption. In this work, we demonstrate an optoelectronic device based on the combination of two-dimensional material and carbon dot with wide bandgap. High-efficient luminescence of carbon dot and extremely large shape anisotropy (>1500) of two-dimensional material with the wide bandgap of >4 eV cooperatively endow the optoelectronic device with multi-functions of optically anisotropic blue-light emission, visible light modulation, wavelength-dependent ultraviolet-light detection as well as blue fluorescent film assemble. This research opens new avenues for constructing multi-function-integrated optoelectronic devices via the combination of nanomaterials with different dimensions.
低维材料由于在一个或多个维度上的纳米级尺寸而表现出独特的量子限制效应和形态,这使得它们与块状材料相比具有独特的物理性质。在所有低维材料中,二维材料因其原子级厚度而具有极大的形状各向异性,因此推测具有很大的光学各向异性吸收。在这项工作中,我们展示了一种基于二维材料和宽带隙碳点组合的光电器件。宽带隙大于4 eV的二维材料的极大形状各向异性(>1500)与碳点的高效发光协同赋予该光电器件光学各向异性蓝光发射、可见光调制、波长依赖的紫外光检测以及蓝色荧光膜组装等多功能。这项研究为通过不同维度纳米材料的组合构建多功能集成光电器件开辟了新途径。