Suppr超能文献

利用航空通量测量评估加利福尼亚圣华金河谷奶制品运营中的甲烷排放。

Methane Emissions from Dairy Operations in California's San Joaquin Valley Evaluated Using Airborne Flux Measurements.

机构信息

Division of Geological and Planetary Sciences, California Institute of Technology, Pasadena, California 91125, United States.

Department of Environmental Science and Policy Management, University of California Berkeley, Berkeley, California 94720, United States.

出版信息

Environ Sci Technol. 2023 Dec 5;57(48):19519-19531. doi: 10.1021/acs.est.3c03940. Epub 2023 Nov 24.

Abstract

State inventories indicate that dairy operations account for nearly half of California's methane budget. Recent analyses suggest, however, that these emissions may be underestimated, complicating efforts to develop emission reduction strategies. Here, we report estimates of dairy methane emissions in the southern San Joaquin Valley (SJV) of California in June 2021 using airborne flux measurements. We find average dairy methane fluxes of 512 ± 178 mg m h from a region of 300+ dairies near Visalia, CA using a combination of eddy covariance and mass balance-based techniques, corresponding to 118 ± 41 kg dairy h. These values estimated during our June campaign are 39 ± 48% larger than annual average estimates from the recently developed VISTA-CA inventory. We observed notable increases in emissions with temperature. Our estimates align well with inventory predictions when parametrizations for the temperature dependence of emissions are applied. Our measurements further demonstrate that the VISTA-CA emission inventory is considerably more accurate than the EPA GHG-I inventory in this region. Source apportionment analyses confirm that dairy operations produce the majority of methane emissions in the southern SJV (∼65%). Fugitive oil and gas (O&G) sources account for the remaining ∼35%. Our results support the accuracy of the process-based models used to develop dairy emission inventories and highlight the need for additional investigation of the meteorological dependence of these emissions.

摘要

州库存数据表明,奶制品生产占加利福尼亚州甲烷预算的近一半。然而,最近的分析表明,这些排放量可能被低估了,这使得制定减排策略的工作变得更加复杂。在这里,我们报告了 2021 年 6 月利用机载通量测量在加利福尼亚州圣华金河谷南部(SJV)估算奶制品甲烷排放量的结果。我们使用涡度相关和基于质量平衡的技术相结合,从加利福尼亚州维塞利亚附近的 300 多家奶制品农场的区域中发现,平均奶制品甲烷通量为 512 ± 178 mg m h,这相当于 118 ± 41 kg 奶制品 h。我们在 6 月的研究期间得出的这些值比最近开发的 VISTA-CA 清单的年平均估计值高出 39 ± 48%。我们发现排放物随温度的升高而显著增加。当应用排放物对温度的依赖关系的参数化时,我们的估算值与清单预测值吻合良好。我们的测量结果进一步表明,在该地区,VISTA-CA 排放清单比 EPA GHG-I 清单准确得多。来源分配分析证实,奶制品生产是 SJV 南部(约 65%)甲烷排放的主要来源。逸散性石油和天然气(O&G)源占其余的约 35%。我们的结果支持了用于开发奶制品排放清单的基于过程的模型的准确性,并强调了需要进一步研究这些排放物对气象的依赖关系。

文献AI研究员

20分钟写一篇综述,助力文献阅读效率提升50倍。

立即体验

用中文搜PubMed

大模型驱动的PubMed中文搜索引擎

马上搜索

文档翻译

学术文献翻译模型,支持多种主流文档格式。

立即体验