Department of Chemistry and KI for the BioCentury, Korea Advanced Institute of Science and Technology (KAIST), Daejeon 34141, Republic of Korea.
Center for Advanced Reaction Dynamics (CARD), Institute for Basic Science (IBS), Daejeon 34141, Republic of Korea.
Int J Mol Sci. 2023 Dec 5;24(24):17135. doi: 10.3390/ijms242417135.
Biological macromolecules, the fundamental building blocks of life, exhibit dynamic structures in their natural environment. Traditional structure determination techniques often oversimplify these multifarious conformational spectra by capturing only ensemble- and time-averaged molecular structures. Addressing this gap, in this work, we extend the application of the single-object scattering sampling (SOSS) method to diverse biological molecules, including RNAs and proteins. Our approach, referred to as "Bio-SOSS", leverages ultrashort X-ray pulses to capture instantaneous structures. In Bio-SOSS, we employ two gold nanoparticles (AuNPs) as labels, which provide strong contrast in the X-ray scattering signal, to ensure precise distance determinations between labeled sites. We generated hypothetical Bio-SOSS images for RNAs, proteins, and an RNA-protein complex, each labeled with two AuNPs at specified positions. Subsequently, to validate the accuracy of Bio-SOSS, we extracted distances between these nanoparticle labels from the images and compared them with the actual values used to generate the Bio-SOSS images. Specifically, for a representative RNA (1KXK), the standard deviation in distance discrepancies between molecular dynamics snapshots and Bio-SOSS retrievals was found to be optimally around 0.2 Å, typically within 1 Å under practical experimental conditions at state-of-the-art X-ray free-electron laser facilities. Furthermore, we conducted an in-depth analysis of how various experimental factors, such as AuNP size, X-ray properties, and detector geometry, influence the accuracy of Bio-SOSS. This comprehensive investigation highlights the practicality and potential of Bio-SOSS in accurately capturing the diverse conformation spectrum of biological macromolecules, paving the way for deeper insights into their dynamic natures.
生物大分子是生命的基本组成部分,在其自然环境中呈现出动态结构。传统的结构测定技术通常通过仅捕获整体和时间平均的分子结构,而过于简化这些多样化的构象谱。为了解决这一差距,在这项工作中,我们将单物体散射采样 (SOSS) 方法扩展应用于包括 RNA 和蛋白质在内的各种生物分子。我们的方法称为“Bio-SOSS”,利用超短 X 射线脉冲捕捉瞬时结构。在 Bio-SOSS 中,我们使用两个金纳米粒子 (AuNP) 作为标记物,它们在 X 射线散射信号中提供强对比度,以确保标记位点之间的精确距离测定。我们生成了 RNA、蛋白质和 RNA-蛋白质复合物的假想 Bio-SOSS 图像,每个图像在指定位置标记有两个 AuNP。随后,为了验证 Bio-SOSS 的准确性,我们从图像中提取这些纳米粒子标记之间的距离,并将其与用于生成 Bio-SOSS 图像的实际值进行比较。具体来说,对于代表性的 RNA(1KXK),在分子动力学快照和 Bio-SOSS 检索之间的距离差异的标准偏差被发现最佳约为 0.2 Å,在最先进的 X 射线自由电子激光设施的实际实验条件下,通常在 1 Å 以内。此外,我们深入分析了各种实验因素,如 AuNP 尺寸、X 射线特性和探测器几何形状,如何影响 Bio-SOSS 的准确性。这项综合研究强调了 Bio-SOSS 在准确捕捉生物大分子多样化构象谱方面的实用性和潜力,为深入了解它们的动态性质铺平了道路。